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Magnetic phase transitions in R/sub 2/Fe/sub 17/ compounds under pressure

机译:R / sub 2 / Fe / sub 17 /化合物在压力下的磁性相变

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The effect of the pressure up to 1.4 GPa on the Curie temperature T/sub c/ in the R/sub 2/Fe/sub 17/ intermetallics with R=Nd, Er and Y was measured using a low field susceptibility technique. The identical character of the temperature dependence of susceptibility X(T) of the R/sub 2/Pe/sub 17/ intermetallics observed at ambient pressure (sharp step-like drop at T/sub c/) is preserved at high pressures only in the case of Nd/sub 2/Fe/sub 17/. Pronounced broadening and splitting of the sharp drop of X(T) was observed in Er/sub 2/Fe/sub 17/ and Y/sub 2/Fe/sub 17/ respectively. The initial pressure slopes of dTc/dp are large and negative for all studied compounds, having nearly the same values (dTc/dp=-36K/GPa for Nd/sub 2/Fe/sub 17/ compound). Our results are discussed from the point of view of the sensitivity of T/sub c/ on the crystal structure, the number of nearest neighbours of Fe atoms and the possible effect of "disordered" structures in the R/sub 2/Fe/sub 17/ intermetallics.
机译:使用低场磁化率技术测量了高达1.4 GPa的压力对R / sub 2 / Fe / sub 17 /金属间化合物中R = Nd,Er和Y的居里温度T / sub c /的影响。 R / sub 2 / Pe / sub 17 /金属间化合物在环境压力下观察到的磁化率X(T)的温度依存性的相同特征(在T / sub c /处出现陡峭的阶梯状下降)仅在高压下保持。 Nd / sub 2 / Fe / sub 17 /的情况。分别在Er / sub 2 / Fe / sub 17 /和Y / sub 2 / Fe / sub 17 /中观察到X(T)急剧下降的明显扩展和分裂。对于所有研究的化合物,dTc / dp的初始压力斜率都大且为负值,几乎具有相同的值(对于Nd / sub 2 / Fe / sub 17 /化合物,dTc / dp = -36K / GPa)。从T / sub c /对晶体结构的敏感性,Fe原子最近邻的数量以及R / sub 2 / Fe / sub中“无序”结构的可能影响的角度讨论了我们的结果。 17 /金属间化合物。

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