Assessment of bias-adjusted PM_2.5 air quality forecasts over the continental United States during 2007

摘要

To develop fine particular matter (PM_2.5) air quality forecasts, a National Air Quality Forecast Capability (NAQFC) system, which linked NOAA's North American Mesoscale (NAM) meteorological model with EPA's Community Multiscale Air Quality (CMAQ) model, was deployed in the developmental mode over the continental United States during 2007. This study investigates the operational use of a bias-adjustment technique called the Kalman Filter Predictor approach for improving the accuracy of the PM_2.5 forecasts at monitoring locations. The Kalman Filter Predictor bias-adjustment technique is a recursive algorithm designed to optimally estimate bias-adjustment terms using the information extracted from previous measurements and forecasts. The bias-adjustment technique is found to improve PM_2.5 forecasts (i.e. reduced errors and increased correlation coefficients) for the entire year at almost all locations. The NAQFC tends to overestimate PM_2.5 during the cool season and underestimate during the warm season in the eastern part of the continental US domain, but the opposite is true for the pacific coast. In the Rocky Mountain region, the NAQFC system overestimates PM_2.5 for the whole year. The bias-adjustment forecasts can quickly (after 2–3 days' lag) adjust to reflect the transition from one regime to the other. The modest computational requirements and systematical improvements in forecast results across all seasons suggest that this technique can be easily adapted to perform bias-adjustment for real-time PM_2.5 air quality forecasts.