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Introduction of amino and rGO into PP nonwoven surface for removal of gaseous aromatic pollutants and particulate matter from air

机译:将氨基和rGO引入PP无纺布表面,以去除空气中的气态芳族污染物和颗粒物

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摘要

Gaseous aromatic pollutants such as benzene, toluene or xylene and particulate matter (PM) from an individual's living environment potentially cause serious and life-threatening health problems. A new bifunctional individual protection material was prepared by grafting polymerization and electrostatic self-assembly method. The individual protection material has a dual function layer consisting of an amino-functionalized nonwoven grafted with dimethylaminoethyl methacrylate (DMAEMA) and a gaseous aromatic pollutant adsorption layer made up of reduced graphene oxide (rGO). The surface composition and structure of materials were obtained by a series of characterization methods. Adsorption and filtration performance for each function layer and double function layer Polypropylene (PP) nonwoven were intensively studied. As indicated by the experiments, the adsorption efficiency of PP-g-DMAEMA/rGO increased with the decreasing oxygen content of GO and increasing the initial concentration of toluene, filter performance and aperture parameters data showed that the surface Zeta potential and pore size had great influence on filtration efficiency of the filter material, the resulting PP nonwoven exhibited prominent multifunctional performance, including a higher adsorption amount (39.1 mg/g) and filter efficiency (72.2%). Consequently, it is expected that the bifunctional PP nonwoven will have potential applications in air purification for the removal of gaseous aromatic pollutants and PM.
机译:个人生活环境中的气态芳香族污染物(例如苯,甲苯或二甲苯)和颗粒物(PM)可能会导致严重且威胁生命的健康问题。通过接枝聚合和静电自组装法制备了一种新型的双功能个体防护材料。单独的保护材料具有双重功能层,该双重功能层由接枝有甲基丙烯酸二甲基氨基乙基酯(DMAEMA)的氨基官能化无纺布和由还原型氧化石墨烯(rGO)构成的气态芳族污染物吸附层组成。材料的表面组成和结构是通过一系列表征方法获得的。对每个功能层和双重功能层的吸附和过滤性能进行了深入研究。实验表明,PP-g-DMAEMA / rGO的吸附效率随GO含氧量的降低和甲苯初始浓度的增加而增加,过滤性能和孔径参数数据表明,表面Zeta势和孔径均很大。通过对过滤材料的过滤效率的影响,所得的PP无纺布表现出突出的多功能性能,包括更高的吸附量(39.1mg / g)和过滤效率(72.2%)。因此,期望双功能PP无纺布将在空气净化中具有潜在的应用,以去除气态芳族污染物和PM。

著录项

  • 来源
    《Applied Surface Science》 |2020年第1期|145631.1-145631.11|共11页
  • 作者单位

    Tiangong Univ State Key Lab Separat Membranes & Membrane Proc N Natl Ctr Int Joint Res Separat Membranes Tianjin 300387 Peoples R China|Tiangong Univ Sch Mat Sci & Engn Tianjin 300387 Peoples R China;

    Tiangong Univ State Key Lab Separat Membranes & Membrane Proc N Natl Ctr Int Joint Res Separat Membranes Tianjin 300387 Peoples R China|Tiangong Univ Sch Mat Sci & Engn Tianjin 300387 Peoples R China|Tiangong Univ Sch Environm Sci & Engn Tianjin 300387 Peoples R China|Tiangong Univ Sch Chem & Chem Engn Tianjin 300387 Peoples R China;

    Tiangong Univ State Key Lab Separat Membranes & Membrane Proc N Natl Ctr Int Joint Res Separat Membranes Tianjin 300387 Peoples R China|Tianjin Engn Ctr Safety Evaluat Water & Safeguard Tianjin 300387 Peoples R China|Tiangong Univ Sch Environm Sci & Engn Tianjin 300387 Peoples R China;

    Tiangong Univ State Key Lab Separat Membranes & Membrane Proc N Natl Ctr Int Joint Res Separat Membranes Tianjin 300387 Peoples R China|Tiangong Univ Sch Chem & Chem Engn Tianjin 300387 Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    rGO; Polypropylene nonwoven; Gaseous aromatic pollutants; Adsorption; PM filtration;

    机译:rGO;聚丙烯无纺布;气态芳香污染物;吸附;PM过滤;

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