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Enhanced dipole-dipole interaction of CdSe/CdS nanocrystal quantum dots inside a planar microcavity

机译:平面微腔内CdSe / CdS纳米晶体量子点的偶极子-偶极相互作用增强

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摘要

The energy transfer (ET) dynamics of closely packed CdSe/CdS nanocrystal quantum dots (NQDs) embedded in a planar microcavity were studied by using time-resolved photoluminescence measurements. An increase of ~20% was observed in the rates of ET from smaller to larger NQDs in the mierocavity as compared with those measured in free space. This behavior was attributed to the enhanced dipole-dipole interactions between donor and acceptor NQDs at the spectral positions of the cavity modes.
机译:通过使用时间分辨光致发光测量研究了嵌入在平面微腔中的紧密堆积的CdSe / CdS纳米晶体量子点(NQD)的能量转移(ET)动力学。与在自由空间中测量的相比,在微腔中,从较小的NQD到较大的NQD,ET的比率增加了约20%。该行为归因于在腔模的光谱位置处的供体和受体NQD之间增强的偶极-偶极相互作用。

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