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Inelastic X-ray scattering measurements of Ⅲ-V multiple quantum wells

机译:Ⅲ-Ⅴ族多量子阱的非弹性X射线散射测量

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摘要

Inelastic X-ray scattering (IXS) on an In_(0.17)Ga_0.83)As/GaAs_(0.8)P_(0.2) multiple quantum well (MQW) superlattice has been conducted to investigate the potential for phonon bottlenecks in low dimensional materials. This work shows that the measured spectra are in good agreement with an adia-batic bond charge model prediction and back-folded phonon modes make large contributions to the broadening of peaks observed in the spectra. The high-lying mode at 45 meV in the MQW is attributed to vibrations of Ga and P and confirmed by both experiment and theory. The acoustic phonons have a dominant contribution from the Ga and As components, and the contribution from InAs is small and only visible at around 29.7 meV. Low energy optical modes resulting from back-folding might be a key to increased electron-phonon coupling in the material system. The suitability of utilizing IXS as a means to investigate phonon modes in low dimensional materials is also discussed.
机译:在In_(0.17)Ga_0.83)As / GaAs_(0.8)P_(0.2)多量子阱(MQW)超晶格上进行了非弹性X射线散射(IXS),以研究低维材料中声子瓶颈的可能性。这项工作表明,测得的光谱与绝热键电荷模型的预测非常吻合,而后折声子模式对光谱中观察到的峰变宽做出了很大贡献。 MQW中45 meV的高空模式归因于Ga和P的振动,并已通过实验和理论确认。声子在Ga和As成分中起主要作用,而InAs的作用很小,仅在29.7 meV附近可见。反折产生的低能光学模式可能是增加材料系统中电子-声子耦合的关键。还讨论了使用IXS作为研究低维材料中声子模的手段的适用性。

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  • 来源
    《Applied Physics Letters》 |2017年第4期|043102.1-043102.5|共5页
  • 作者单位

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    University of New South Wales, Sydney 2052, Australia;

    Research and Utilization Division, Japan Synchrotron Radiation Research Institute, SPring-8,1-1-1 Kouto, Sayo, Hyogo 679-5198, Japan;

    Research and Utilization Division, Japan Synchrotron Radiation Research Institute, SPring-8,1-1-1 Kouto, Sayo, Hyogo 679-5198, Japan;

    Department of Electrical Engineering and Information Systems, School of Engineering,The University of Tokyo, Tokyo 113-8656, Japan;

    Materials Dynamics Laboratory, RIKEN SPring-8 Center, Sayo, Hyogo 679-5148, Japan;

    University of New South Wales, Sydney 2052, Australia;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
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