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Human Health Risk Assessment of 16 Priority Polycyclic Aromatic Hydrocarbons in Soils of Chattanooga Tennessee USA

机译:田纳西州田纳西州的16个优先多环芳烃烃的人体健康风险评估

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摘要

South Chattanooga has been home to foundries, coke furnaces, chemical, wood preserving, tanning and textile plants for over 100 years. Most of the industries were in place before any significant development of residential property in the area. During the 1950s and 1960s, however, the government purchased inexpensive property and constructed public housing projects in South Chattanooga. Many neighborhoods that surround the Chattanooga Creek were previous dumping grounds for industry. Polycyclic aromatic hydrocarbons (PAHs) comprised the largest component of the dumping and airborne industrial emissions. To address the human exposure to these PAHs, a broad study of South Chattanooga soil contaminant concentrations was conducted on 20 sites across the city. Sixteen priority pollutant PAHs were quantified at two depths (0-10cm and 10-20cm) and compared against reference site soils, as well as to soils from industrially-impacted areas in Germany, China, and the US. From these data, the probability that people would encounter levels exceeding EPA Residential Preliminary Remediation Goals (PRG) was calculated. Results indicate that South Chattanooga soils have relatively high concentrations of total PAHs, specifically Benzo[a]pyrene (B[a]P). These high concentrations of B[a]P were somewhat ubiquitous in South Chattanooga. Indeed, there is a high probability (88%) of encountering soil in South Chattanooga that exceeds the EPA PRG for B[a]P. However, there is a low probability (15%) of encountering a site with ∑PAHs exceeding EPA PRG guidelines.
机译:南查塔努加(South Chattanooga)拥有铸造厂,炼焦炉,化学制品,木材防腐,鞣革厂和纺织厂,已有100多年的历史了。在该地区住宅物业出现任何重大发展之前,大多数行业都已经存在。然而,在1950年代和1960年代期间,政府在南查塔努加购买了廉价房地产并建造了公共住房项目。查塔努加河(Chattanooga Creek)周围的许多社区以前都是工业的垃圾场。多环芳烃(PAHs)是倾倒和空气传播的工业排放中最大的组成部分。为了解决人类暴露于这些多环芳烃的问题,在整个城市的20个地点对南查塔努加土壤污染物的浓度进行了广泛的研究。在两个深度(0-10cm和10-20cm)处对16种优先污染物PAHs进行了定量,并与参考地点的土壤以及德国,中国和美国的工业影响区的土壤进行了比较。根据这些数据,计算出人们遇到超过EPA住宅初步补救目标(PRG)的可能性。结果表明,南查塔努加土壤中的总PAH含量相对较高,特别是苯并[a] re(B [a] P)。这些高浓度的B [a] P在南查塔努加市普遍存在。实际上,在南查塔努加遇到土壤的可能性很高(88%),超过了B [a] P的EPA PRG。但是,遇到∑PAH超过EPA PRG准则的站点的可能性很小(15%)。

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