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Deterministic strain-induced arrays of quantum emitters in a two-dimensional semiconductor

机译:二维半导体中确定性的应变诱导量子发射器阵列

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摘要

An outstanding challenge in quantum photonics is scalability, which requires positioning of single quantum emitters in a deterministic fashion. Site positioning progress has been made in established platforms including defects in diamond and self-assembled quantum dots, albeit often with compromised coherence and optical quality. The emergence of single quantum emitters in layered transition metal dichalcogenide semiconductors offers new opportunities to construct a scalable quantum architecture. Here, using nanoscale strain engineering, we deterministically achieve a two-dimensional lattice of quantum emitters in an atomically thin semiconductor. We create point-like strain perturbations in mono- and bi-layer WSe2 which locally modify the band-gap, leading to efficient funnelling of excitons towards isolated strain-tuned quantum emitters that exhibit high-purity single photon emission. We achieve near unity emitter creation probability and a mean positioning accuracy of 120±32 nm, which may be improved with further optimization of the nanopillar dimensions.
机译:量子光子学中的一个巨大挑战是可伸缩性,它要求以确定性的方式放置单个量子发射器。尽管通常会损害相干性和光学质量,但在已建立的平台(包括钻石和自组装量子点中的缺陷)的站点定位方面已经取得了进展。分层过渡金属二卤化半导体中单量子发射器的出现为构建可扩展的量子体系结构提供了新的机会。在这里,我们使用纳米级应变工程,确定性地在原子薄的半导体中实现了量子发射器的二维晶格。我们在单层和双层WSe2中创建点状应变摄动,可局部修改带隙,从而将激子有效地漏斗到表现出高纯度单光子发射的孤立的应变调谐量子发射器。我们实现了近乎统一的发射器创建概率,平均定位精度为120±32 nm,可以通过进一步优化纳米柱尺寸来提高。

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