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Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators

机译:通过手征性硅环共振器定制碳纳米管的光学性质

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摘要

Semiconducting single walled carbon nanotubes (s-SWNT) have an immense potential for the development of active optoelectronic functionalities in ultra-compact hybrid photonic circuits. Specifically, s-SWNT have been identified as a very promising solution to implement light sources in the silicon photonics platform. Still, two major challenges remain to fully exploit the potential of this hybrid technology: the limited interaction between s-SWNTs and Si waveguides and the low quantum efficiency of s-SWNTs emission. Silicon micro-ring resonators have the potential capability to overcome these limitations, by providing enhanced light s-SWNT interaction through resonant light recirculation. Here, we demonstrate that Si ring resonators provide SWNT chirality-wise photoluminescence resonance enhancement, releasing a new degree of freedom to tailor s-SWNT optical properties. Specifically, we show that judicious design of the micro-ring geometry allows selectively promoting the emission enhancement of either (8,6) or (8,7) SWNT chiralities present in a high-purity polymer-sorted s-SWNT solution. In addition, we present an analysis of nanometric-sized silicon-on-insulator waveguides that predicts stronger light s-SWNT interaction for transverse-magnetic (TM) modes than for conventionally used transverse-electric (TE) modes.
机译:半导体单壁碳纳米管(s-SWNT)具有开发超紧凑型混合光子电路中有源光电功能的巨大潜力。特别是,s-SWNT已被认为是在硅光子学平台中实现光源的非常有前途的解决方案。尽管如此,充分利用这种混合技术的潜力仍然存在两个主要挑战:s-SWNT和Si波导之间的相互作用有限以及s-SWNT发射的量子效率低。硅微环谐振器具有潜在的能力,可以通过谐振光再循环提供增强的光s-SWNT相互作用来克服这些限制。在这里,我们证明了硅环谐振器提供了SWNT手性方向的光致发光谐振增强,释放了一个新的自由度来调整s-SWNT光学特性。具体而言,我们表明,微环几何结构的明智设计可以选择性地促进高纯度聚合物分类的s-SWNT解决方案中存在的(8,6)或(8,7)SWNT手性的发射增强。此外,我们提出了一种对纳米尺寸的绝缘体上硅波导的分析,该分析预测与传统使用的横向电(TE)模式相比,横向磁(TM)模式的光s-SWNT相互作用更强。

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