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Efficient metal halide perovskite light-emitting diodes with significantly improved light extraction on nanophotonic substrates

机译:高效的金属卤化物钙钛矿发光二极管在纳米光子衬底上的光提取显着改善

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摘要

Metal halide perovskite has emerged as a promising material for light-emitting diodes. In the past, the performance of devices has been improved mainly by optimizing the active and charge injection layers. However, the large refractive index difference among different materials limits the overall light extraction. Herein, we fabricate efficient methylammonium lead bromide light-emitting diodes on nanophotonic substrates with an optimal device external quantum efficiency of 17.5% which is around twice of the record for the planar device based on this material system. Furthermore, optical modelling shows that a high light extraction efficiency of 73.6% can be achieved as a result of a two-step light extraction process involving nanodome light couplers and nanowire optical antennas on the nanophotonic substrate. These results suggest that utilization of nanophotonic structures can be an effective approach to achieve high performance perovskite light-emitting diodes.
机译:钙钛矿金属卤化物已成为发光二极管的有前途的材料。过去,主要通过优化有源注入层和电荷注入层来改善设备的性能。然而,不同材料之间的大的折射率差限制了整个光提取。本文中,我们在纳米光子衬底上制造了高效的甲基铵溴化铅发光二极管,其最佳器件外部量子效率为17.5%,约为基于该材料系统的平面器件记录的两​​倍。此外,光学建模表明,由于在纳米光子基板上进行了两步光提取过程,其中包括纳米圆顶光耦合器和纳米线光学天线,因此可以实现73.6%的高光提取效率。这些结果表明,利用纳米光子结构可以是实现高性能钙钛矿发光二极管的有效方法。

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