Vibrational Coherence Decay in Metal Carbonyls: Solvent Dependence of Coherence Lifetimes Studied with MDIR

摘要

Multidimensional infrared spectra of a metal carbonyl in different solvents are presented as a function of the waiting time, t_2. The evolution of each peak is related to excited-state coherences and the relative correlation between excited state vibrational energies.