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Near-Field Scanning Magneto-Optical Spectroscopy of Wigner Molecules

机译:Wigner分子的近场扫描磁光学光谱

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We study the emission spectra of single self-organized InP/GaInP QDs (size 100-220 nm) using high-spatial-resolution, low-temperature (5K) near-field scanning optical microscope (NSOM) operating at magnetic field strength B=0-10T. The dots contain up to twenty electrons and represent natural Wigner molecules (WM). We observed vibronic-type shake-up structure in single electron QDs manifesting formation of two electron (2e) WM in photo-excited state. We found that relative intensities of the shake-up components described well by vibronic Frank-Condon factors giving for dots having parabolic confinement energy hω_0=1.2-4 meV molecule bond lengths 40-140 nm. We used measurements of magnetic-field-induced shifts to distinguish emission of 2e-WM and singly charged exciton (trion). We also observed magnetic-field-induced molecular-droplet transition for two electron dot, emitting through doubly charge exciton (tetron) at zero magnetic field.
机译:我们使用高空间分辨率,低温(5K)近场扫描光学显微镜(NSOM)研究单一自组织INP / GAIPP QDS(尺寸100-220nm)的发射光谱法在磁场强度B = 0-10t。该点最多包含20个电子,代表天然的Wigner分子(WM)。我们观察了在光激发态中的单电子QD中的振动式振动结构表现为两种电子(2E)WM的形成。我们发现,由抛物线限制能量Hω_0= 1.2-4MEV分子键合长度为40-140nm的抛光坦克 - 坦克因子,所以通过振动坦率的组件的相对强度描述了很好的抛光伞菌。我们使用磁场诱导的变化的测量来区分2E-WM和单电压的激子(TRION)的发射。我们还观察到磁场诱导的两个电子点的分子液滴转变,在零磁场下通过双电荷激子(Tetron)发射。

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