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Influence of Hydrodynamics on Relaxation Time of Dynamics in Colloidal Crystal

机译:流体动力学对胶体晶体动力学放松时间的影响

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We analyzed particle motions in colloidal crystals by digital video microscopy, and obtained the dispersion relations of amplitude and relaxation time for normal relaxation modes of particle dynamics. Because the observed crystals were soft, the soft mode which had larger amplitude and longer relaxation time appeared in -M. Such soft mode, however, could not be reproduced at all by a simple overdamped Langevin theory in which the hydrodynamic interaction and long-range interaction were not incorporated. Therefore we attempted to introduce the influence of flow into the equation of motion by using the Oseen tensor. The results of the modified model were in quantitative agreement with the experimental results. We also found that it was essential to consider the negative force constant between 3rd-nearest neighbor particles for explaining the soft mode.
机译:通过数字视频显微镜分析胶体晶体中的颗粒运动,并获得了粒子动力学正常松弛模式的幅度和弛豫时间的色散关系。因为观察到的晶体柔软,所以具有较大幅度和更长的松弛时间的软模式出现在-M中。然而,这种软模式根本不能通过简单的过度透过的Langevin理论来再现,其中不包含流体动力相互作用和远程相互作用。因此,我们试图通过使用OSEEN张量引入流入运动方程的影响。修改模型的结果与实验结果有定量协议。我们还发现,对于解释软模式,必须考虑第三邻域粒子之间的负力常数。

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