Pulse-Fluence-Specified Optimal Control Simulation with Applications to Molecular Orientation and Spin-Isomer-Selective Molecular Alignment

摘要

We propose an optimal control simulation with specified pulse fluence and amplitude. The simulation is applied to the orientation control of CO molecules to examine the optimal combination of THz and laser pulses, and to discriminate nuclear-spin isomers of ~(14)N_2 as spatially anisotropic distributions.