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Glass transition in a two-dimensional system of magnetic colloids

机译:磁性胶体二维系统中的玻璃过渡

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We describe experiments on binary mixtures of superparamagnetic colloidal particles confined by gravity to a flat horizontal water-air interface. The colloids repel each other because of their magnetic dipole moments induced by a vertical external magnetic field B. By tuning B, the effective temperature of the system can be adjusted over several orders of magnitude. Particle coordinates are monitored by video-microscopy over more than five decades in time. Measured radial pair-distribution functions g(r) and mean-square displacements illustrate that this system is an ideal model of a two-dimensional (2D) glass former. We find that the effects of small amounts of aggregated particles only weakly affect the averaged structure and dynamics. Locally, a small number of elementary structural elements are observed each characterized by a special triangular shape. These triangles arrange in dense mostly space-filling arrays and account for the essential features of g(r). The long-time α-relaxation is related to drifts of arrays as well as erosion due to single particle and collective hopping events.
机译:我们描述了通过重力限制的超顺磁性颗粒的二元混合物的实验,以平坦的水平水空气界面。由于其垂直外部磁场B诱导的磁性偶极矩,胶体彼此互相排斥。通过调谐B,可以在几个数量级上调整系统的有效温度。粒子坐标通过视频显微镜监测超过五十年的时间。测量的径向对分配功能G(R)和均方位移说明该系统是二维(2D)玻璃前的理想模型。我们发现少量聚集颗粒的影响仅弱地影响平均结构和动力学。在本地,观察到少量的基本结构元件,每个结构元素的特征在于特殊的三角形形状。这些三角形布置在密集的空间填充阵列中,并考虑到g(r)的基本特征。长时间α-松弛与阵列的漂移以及由于单个粒子和集体跳跃事件而导致的侵蚀。

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