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Saturation of Dye Solution in Principal Channel by Using Two Light Fields

机译:使用两个光场在主通道中的染料溶液饱和

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A cubic nonlinearity of dye solution can be taken into consideration to study many nonlinear phenomena, such as phase conjugation, holography, amplification [1,2, 5, 6 and 7]. Nonlinear processes strongly depend on intensity and frequency of radiations involved in these processes. A dye solution can be modeled by a typical three-level configuration (S0-S1-S2) , for which the transitions of molecules in principal channel (SO-S1) are realized by the light fields of intensity I12 at frequency ω0. At the same time, light fields with intensity I23 at frequency ω interact with excited molecules to realize their transitions in excited channel (S1-S2). For this model, the conditions of phase response saturation are determined in principal channel. The saturation of phase response of dye solution in principal channel (S0-S1) is realized at saturation intensity I_(12)~(saT) , decreasing with increasing of radiation intensity in excited channel I_(23). The saturation intensity I_(12)~(saT) has its optimum (minimum) values when the frequency of light fields in principal channel is tuned with Stokes shift from the centre of principal absorption band. In addition, the saturation intensity I_(12)~(saT) has its optimum when the radiations in excited channel have enough big intensity I23 and a frequency tuning with anti-Stokes shift from centre of absorption excited band.
机译:可以考虑染料溶液的立方非线性,以研究许多非线性现象,例如相位缀合,全息,扩增[1,2,5,6和7]。非线性过程强烈取决于这些过程中涉及的辐射的强度和频率。染料溶液可以通过典型的三级配置(S0-S1-S2)进行建模,其中主要通道(SO-S1)中的分子转变由频率ω0处的强度I12的光场实现。同时,频率ω处具有强度I23的光场与激发分子相互作用,以实现它们在激发通道(S1-S2)中的转换。对于该模型,阶段响应饱和的条件在主信道中确定。在主通道(S0-S1)中染料溶液相响应的饱和度在饱和强度I_(12)〜(SAT)中实现,随着激励通道I_(23)中的辐射强度的增加而降低。当主通道中的光场的频率随着主体吸收带的中心调谐时,饱和度强度I_(12)〜(SAT)具有其最佳(最小)值。另外,饱和强度I_(12)〜(SAT)当激发通道中的辐射具有足够的大强度I23和频率调谐的饱和度强度I_(SAT)具有其最佳状态,并且使用反斯托克斯从吸收激发带的中心移动。

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