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Direct numerical simulation of reactive mixing in a T-shaped micro-reactor

机译:T形微反应器中反应混合的直接数值模拟

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The large area-to-volume ratio of micro-reactors gives prospect of better yield and selectivity than for conventional designs, since diffusive fluxes of mass and heat in micro-devices scale with the area, while the rate of changes corresponding to sources and sinks are proportional to the volume. Indeed, theoretical considerations of the scaling behavior support the fact that micro-reactors allow for faster chemical reactions and provide better thermal control; cf., e.g., [1]. For applications in Chemical Reaction Engineering, the mixing of chemical species is of special interest, since it is an essential condition for chemical reactions to occur. Avoiding large pressure drops, laminar flow fields with secondary flows are chosen to increase the contact area between the inflowing educts. In this laminar but complex flow, the mixing state is determined by the interplay of convective and diffusive transport phenomena and, hence, a thorough CFD-simulation of yield and selectivity of such a reacting flow requires the resolution of the finest length scales of both the velocity and the concentration field. In order to reduce the numerical complexity we employ a simplified mathematical model of the relevant convection-diffusion-reaction equations similar to the parabolized Navier-Stokes system.
机译:微量反应器的大面积体积比具有比传统设计更好的产量和选择性的前景,因为微量器件与该区域的微型器件尺度的弥散性和热量,而对应于源和水槽的变化率与体积成比例。实际上,缩放行为的理论考虑因素支持微反应器允许更快的化学反应并提供更好的热控制; CF.,例如[1]。对于化学反应工程中的应用,化学物质的混合具有特殊兴趣,因为它是将化学反应发生的必要条件。避免大压降,选择具有二次流动的层流场,以增加充气变差之间的接触面积。在该层状但复杂的流动中,混合状态由对流和漫射传输现象的相互作用决定,因此,这种反应流的产量和选择性的彻底CFD模拟需要分辨率的最低长度速度和浓度场。为了降低数值复杂性,我们采用类似于抛物化的Navier-Stokes系统的相关对流扩散反应方程的简化数学模型。

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