首页> 外文会议>International conference on phenomena in ionized gases;ICPIG 2009 >Diagnostic Based Modeling for Determining Absolute Atomic Oxygen Densities in Radio-Frequency Atmospheric Pressure Helium-Oxygen Plasmas
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Diagnostic Based Modeling for Determining Absolute Atomic Oxygen Densities in Radio-Frequency Atmospheric Pressure Helium-Oxygen Plasmas

机译:基于诊断的模型确定射频大气压氦氧等离子体中的绝对原子氧密度

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Absolute atomic oxygen ground state densities in a radio-frequency driven atmospheric pressure plasma jet, operated in a helium-oxygen mixture, are determined using diagnostic based modeling. One-dimensional numerical simulations of the electron dynamics are combined with time integrated optical emission spectroscopy. The population dynamics of the upper O 3p~3P (λ= 844 ran) atomic oxygen state is governed by direct electron-impact excitation, dissociative excitation, radiation losses, and collisional-induced quenching. Absolute values for atomic oxygen densities are obtained through comparison with the upper Ar 2p_1 (λ= 750.4 nm) state. Results for spatial profiles and power variations are presented and show excellent quantitative agreement with independent two-photon absorption laser-induced fluorescence measurements.
机译:使用基于诊断的模型确定在氦气-氧气混合物中运行的射频驱动大气压等离子体射流中的绝对原子氧基态密度。电子动力学的一维数值模拟与时间积分光发射光谱法相结合。上部O 3p〜3P(λ= 844 ran)原子氧态的种群动力学受直接电子碰撞激发,离解激发,辐射损失和碰撞诱导猝灭的控制。通过与较高的Ar 2p_1(λ= 750.4 nm)状态进行比较,获得原子氧密度的绝对值。提出了空间分布和功率变化的结果,并显示了与独立的双光子吸收激光诱导的荧光测量结果极好的定量一致性。

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