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Coarse aerosol particle size and shape characteristics near ground level of Shijiazhuang city, China

机译:石家庄市近地面粗粒气溶胶的粒径和形状特征

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摘要

This research sampled subaerial ambient coarse aerosol particles (>2μm of equivalent area diameter) in the typical air polluted city of Shijiazhuang to measure the particle size distribution and shape characteristics by the analyzer of CIS-50 and the scan electronic microscope of S-570 in the non-heating period and heating period respectively. The results show that the coarse aerosol particle size distribution mode is 2~4μm in the non-heating period and 3-5μm in the heating period, with the size range of 0.8~120μm, mostly under 10μm; and the square or square like particle shape is dominant, the sphere like lesser, the acute-angle and lathy shape sparse. There exist particle size distribution and shape characteristics differences in the non-heating period and heating period influenced greatly by the ground coal combustion emission and windblown dust In the heating period, particle size average increases by 53.2%, principally in the size range of 5~10μm, and 20~50μm secondly. Meanwhile, the particle number of quasi-round & round shape group and those with convex-concave fractal edge increase obviously. These quasi-round particles are agglomerate derived from combustion in the SEM images. The relationship between particle size and shape is demonstrated by that the percentage of PM5 and the particle number of the quasi-square & square shape group are positively correlative with r of 0.9458; quasi-round & round shape group negatively correlative with r of -0.9726 respectively.
机译:本研究在典型的空气污染城市石家庄采样了大气环境下的粗颗粒气溶胶颗粒(当量面积直径大于2μm),通过CIS-50分析仪和S-570扫描电子显微镜在石家庄市测量了颗粒尺寸分布和形状特征。分别为非加热期和加热期。结果表明:非加热期粗颗粒气溶胶粒径分布模式为2〜4μm,加热期为3-5μm,粒径分布范围为0.8〜120μm,多数在10μm以下。正方形或正方形的颗粒形状占优势,球形的较小,锐角和板条状的稀疏。地煤燃烧排放和风尘对非采暖期和采暖期粒度分布和形状特征的差异较大。采暖期粒度平均增加53.2%,主要在5〜5的范围内。 10μm,其次为20〜50μm。同时,准圆形和圆形组以及具有凹凸面分形边缘的颗粒数明显增加。这些准圆形粒子是在SEM图像中燃烧产生的团聚体。颗粒大小与形状之间的关系表明,PM5的百分含量与准方形和方形组的颗粒数呈正相关,r为0.9458。准圆形和圆形组分别与-0.9726的r呈负相关。

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