Ultrafast Aqueous Bimolecular Acid-Base Proton Transfer:from Direct Exchange to Sequential Hopping

机译：超快速的水基双分子酸基质子转移：从直接交换到顺序跳跃

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We explore the aqueous neutralization reaction between a photoacid ROH andrncarboxylate basesrn–OOCR' and show that proton transfer in loose complexes (ROH..H2O..–OOCR')rnoccurs through intermediate water molecules in a sequential von Grotthuss type fashion.

机译：我们探索了光酸ROH和羧基羧酸碱基rn-OOCR'之间的水中和反应，并表明在松散配合物（ROH..H2O ..- OOCR'）中的质子转移以顺序von Grotthuss型方式通过中间水分子发生。

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来源
《15th International conference on ultrafast phenomena topical meeting and tabletop exhibit (technical digest)》|2006年|1-3|共3页
会议地点 Pacific Grove CA (US)
作者
O. F. Mohammed; J. Dreyer; E. T. J. Nibbering; D. Pines; E. Pines;
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作者单位

Max Born Institut fuer Nichtlineare Optik und Kurzzeitspektroskopie, Max Born Strasse 2A, D-12489 Berlin, Germany;

Max Born Institut fuer Nichtlineare Optik und Kurzzeitspektroskopie, Max Born Strasse 2A, D-12489 Berlin, Germany;

Max Born Institut fuer Nichtlineare Optik und Kurzzeitspektroskopie, Max Born Strasse 2A, D-12489 Berlin, Germany;

Department of Chemistry, Ben-Gurion University of the Negev, P.O.B. 653, Beersheva 84105, Israel;

Department of Chemistry, Ben-Gurion University of the Negev, P.O.B. 653, Beersheva 84105, Israel;

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原文格式 PDF
正文语种 eng
中图分类超声学;
关键词
(320.7150) Ultrafast spectroscopy; (300.6250) Spectroscopy, condensed matter; (300.6340) Spectroscopy,rninfrared;

机译：（320.7150）超快速光谱法；（300.6250）光谱学，冷凝物；（300.6340）红外光谱;

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专利

1. Aqueous bimolecular proton transfer in acid-base neutralization [J] . Mohammed OF, Pines D, Pines E, Chemical Physics: A Journal Devoted to Experimental and Theoretical Research Involving Problems of Both a Chemical and Physical Nature . 2007,第1a3期

机译：酸碱中和中的双分子水质子转移
2. Real Time Quantification of Ultrafast Photoinduced Bimolecular Electron Transfer Rate: Direct Probing of the Transient Intermediate [J] . Mukherjee Puspal, Biswas Somnath, Sen Pratik The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical . 2015,第34期

机译：实时定量的超快光致双分子电子转移速率：瞬态中间体的直接探测。
3. Ab Initio and Density Functional Theory Study of Keto–Enol Equilibria of Deltic Acid in Gas and Aqueous Solution Phase: A Bimolecular Proton Transfer Mechanism [J] . Jovan M. Tadić † and Lai Xu ‡ The Journal of Organic Chemistry . 2012,第19期

机译：气相和水溶液相中delite酸的酮-烯醇平衡的从头算和密度泛函理论研究：双分子质子转移机理
4. Ultrafast Aqueous Bimolecular Acid-Base Proton Transfer: from Direct Exchange to Sequential Hopping [C] . International conference on ultrafast phenomena topical meeting and tabletop exhibit . 2006

机译：超快水性双分子酸碱酸碱转移：从直接交换到顺序跳跃
5. Bimolecular encounters: Acid-base and/or electron transfer in ruthenium (II) complexes. Experiment and theory. [D] . Kowalczyk, Marta. 2013

机译：双分子相遇：钌（II）配合物中的酸碱和/或电子转移。实验与理论。
6. Salicylic Acid and Analogs: Diamagnetic Chemical Exchange Saturation Transfer (diaCEST) Magnetic Resonance Imaging (MRI) Contrast Agents with Highly Shifted Exchangeable Protons [O] . Xing Yang, Xiaolei Song, Yuguo Li, -1

机译：水杨酸和类似物：具有高度可交换质子的反磁性化学交换饱和转移（diaCEST）磁共振成像（MRI）造影剂
7. Model-free Investigation of Ultrafast Bimolecular Chemical Reactions: Bimolecular Photo Induced Electron Transfer [O] . Bernhard Lang, Arnulf Rosspeintner, Eric Vauthey 2013

机译：无氮屠宰分散化学反应的无模型调查：双分子照片诱导电子转移

Ultrafast Aqueous Bimolecular Acid-Base Proton Transfer:from Direct Exchange to Sequential Hopping

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