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Microporous crystalline material (ITQ-19) with laminar characteristics, preparation method and use thereof as a catalyst in the catalytic conversion of organic compounds
Microporous crystalline material (ITQ-19) with laminar characteristics, preparation method and use thereof as a catalyst in the catalytic conversion of organic compounds
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机译:具有层流特性的微孔晶体材料(ITQ-19),制备方法及其在有机化合物催化转化中的催化剂用途
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摘要
The invention relates to a novel microporous crystalline material ITQ-19 used in the catalytic conversion of organic compounds, such as, for example, the dewaxing and isodewaxing of paraffins and the disproportionation of toluene. Said material has a characteristic X-ray diffractogram, a high absorption capacity and the empirical formula x(M1/nXO2):yYO2:(1−y)SiO2 wherein x has a value less than 0.2; y has a value less than 0.1; M is at least an inorganic cation with a +n charge; X is at least a chemical element having oxidation state +3, preferably selected among Al, Ga, B, Cr, Fe; Y is at least a chemical element with oxidation stated +4, preferably selected among Ge, Ti, Sn, V. The inventive material can be obtained by means of a preparation process involving the use of one or more organic additives in a reaction mix which is crystallized by heating.
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机译:本发明涉及一种新型的微孔晶体材料ITQ-19,其用于有机化合物的催化转化,例如,链烷烃的脱蜡和异脱蜡以及甲苯的歧化。所述材料具有特征X射线衍射图,高吸收能力和经验公式x(M 1 / n Sub> XO 2 Sub>):yYO 2 Sub > :( 1-y)SiO 2 Sub>其中,x的值小于0.2; y的值小于0.1; M至少是带+ n电荷的无机阳离子; X为至少具有+3氧化态的化学元素,优选选自Al,Ga,B,Cr,Fe; Y至少是氧化表示为+4的化学元素,优选选自Ge,Ti,Sn,V。本发明的材料可以通过包括在反应混合物中使用一种或多种有机添加剂的制备方法来获得。通过加热而结晶。
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