Stable dispersions of single and multiple graphene layers in solution

摘要

A method for producing colloidal graphene dispersions comprises the steps of: (i) stirring graphite oxide in an aqueous dispersion medium to form a dispersion; (ii) determining if the dispersion is optically clear in a light microscope at 1000 fold magnification after 1 to 5 hours of stirring, and, if not clear, removing any undissolved impurities in the dispersion, in order to form a colloidal graphene oxide dispersion, or a multi-graphene oxide dispersion, that is optically clear in a light microscope at 1000 fold magnification; and (iii) thermally reducing the graphene oxide, or multi-graphene oxide, in dispersion in the aqueous dispersion medium at a temperature between 120° C. and 170° C. under pressure in order to ensure that the dispersion medium is not evaporated to form a stable colloidal graphene dispersion or a stable multi-graphene dispersion. Using the method used for the preparation of the starting dispersion a graphene or a multi-graphene dispersion is obtained that can be further processed to multi-graphene with larger inter-planar distances than graphite. Such dispersions and multi-graphenes are suitable materials in the manufacturing of rechargeable lithium ion batteries.