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A classical treatment of optical tunneling in plasmonic gaps: extending the quantum corrected model to practical situations

机译:等离子体间隙中光隧穿的经典处理:将量子校正模型扩展到实际情况

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The optical response of plasmonic nanogaps is challenging to address when the separation between the two nanoparticles forming the gap is reduced to a few nanometers or even subnanometer distances. We have compared results of the plasmon response within different levels of approximation, and identified a classical local regime, a nonlocal regime and a quantum regime of interaction. For separations of a few Angstroms, in the quantum regime, optical tunneling can occur, strongly modifying the optics of the nanogap. We have considered a classical effective model, so called Quantum Corrected Model (QCM), that has been introduced to correctly describe the main features of optical transport in plasmonic nanogaps. The basics of this model are explained in detail, and its implementation is extended to include nonlocal effects and address practical situations involving different materials and temperatures of operation.
机译:当形成间隙的两个纳米颗粒之间的距离减小到几纳米甚至亚纳米距离时,等离子体纳米间隙的光学响应难以解决。我们比较了不同近似水平下等离激元响应的结果,并确定了相互作用的经典局域体系,非局域体系和量子体系。对于几埃的分离,在量子状态下会发生光隧道效应,从而极大地改变了纳米间隙的光学特性。我们考虑了一个经典的有效模型,即所谓的量子校正模型(QCM),该模型已被引入以正确描述等离激元纳米间隙中光学传输的主要特征。详细说明了该模型的基础,并将其实现扩展到包括非局部效应,并解决了涉及不同材料和操作温度的实际情况。

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