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首页> 外文期刊>Angewandte Chemie >Highly Efficient Porous Carbon Electrocatalyst with Controllable N‐Species Content for Selective CO2 Reduction
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Highly Efficient Porous Carbon Electrocatalyst with Controllable N‐Species Content for Selective CO2 Reduction

机译：具有可控N型含量的高效多孔碳电催化剂，可减少选择性CO2含量

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Abstract > We report a straightforward strategy to design efficient N doped porous carbon (NPC) electrocatalyst that has a high concentration of easily accessible active sites for the CO <sub>2</sub> reduction reaction (CO <sub>2</sub> RR). The NPC with large amounts of active N (pyridinic and graphitic N) and highly porous structure is prepared by using an oxygen‐rich metal–organic framework (Zn‐MOF‐74) precursor. The amount of active N species can be tuned by optimizing the calcination temperature and time. Owing to the large pore sizes, the active sites are well exposed to electrolyte for CO <sub>2</sub> RR. The NPC exhibits superior CO <sub>2</sub> RR activity with a small onset potential of ?0.35?V and a high faradaic efficiency (FE) of 98.4?% towards CO at ?0.55?V vs. RHE, one of the highest values among NPC‐based CO <sub>2</sub> RR electrocatalysts. This work advances an effective and facile way towards highly active and cost‐effective alternatives to noble‐metal CO <sub>2</sub> RR electrocatalysts for practical applications. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 我们举报了设计有效的N掺杂多孔碳（NPC）电催化剂的直接策略，该电催化剂具有高浓度的易于访问的活性部位 <sub> 2 </ sub> 还原反应（CO <sub> 2 </ sub> RR）。通过使用富氧金属 - 有机骨架（Zn-MOF-74）前体，制备具有大量活性N（吡啶碱和石墨N）和高度多孔结构的NPC。可以通过优化煅烧温度和时间来调谐有源N种的量。由于孔隙尺寸大，活性位点很好地暴露于CO的电解质 <sub> 2 </ sub> rr。 NPC展示优越的公司 <sub> 2 </ sub> RR活动的发病潜力的较小潜力，朝向CO的CO.0.55？V与RHE，基于NPC的CO之间的最高值之​​一 <sub> 2 </ sub> rr电催化剂。这项工作提高了对高贵金属公司的高度积极和经济高效的替代方案的有效和便利的方式 <sub> 2 </ sub> 用于实际应用的RR电催化剂。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第8期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ye Lin&option=202" target="_blank" rel="nofollow">Ye Lin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ying Yiran&option=202" target="_blank" rel="nofollow">Ying Yiran;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Dengrong&option=202" target="_blank" rel="nofollow">Sun Dengrong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Zhouyang&option=202" target="_blank" rel="nofollow">Zhang Zhouyang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fei Linfeng&option=202" target="_blank" rel="nofollow">Fei Linfeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wen Zhenhai&option=202" target="_blank" rel="nofollow">Wen Zhenhai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qiao Jinli&option=202" target="_blank" rel="nofollow">Qiao Jinli;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Haitao&option=202" target="_blank" rel="nofollow">Huang Haitao;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Applied PhysicsThe Hong Kong Polytechnic UniversityHung Hom Kowloon Hong Kong China;</p> <p>Department of Applied PhysicsThe Hong Kong Polytechnic UniversityHung Hom Kowloon Hong Kong China;</p> <p>Department of Chemical EngineeringPohang University of Science and Technology (POSTECH)Nam-gu Pohang-Si Gyungsangbuk-do 37673 South Korea;</p> <p>School of Materials Science and EngineeringNanchang UniversityNanchang Jiangxi 330031 China;</p> <p>Department of Applied PhysicsThe Hong Kong Polytechnic UniversityHung Hom Kowloon Hong Kong China;</p> <p>Fujian Provincial Key Laboratory of NanomaterialsChinese Academy of SciencesFuzhou Fujian 350002 P. R. China;</p> <p>College of Environmental Science and EngineeringDonghua UniversityShanghai 201620 China;</p> <p>Department of Applied PhysicsThe Hong Kong Polytechnic UniversityHung Hom Kowloon Hong Kong China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=CO2 reduction&option=203" rel="nofollow">CO2 reduction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysis&option=203" rel="nofollow">electrocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hierarchically porous materials&option=203" rel="nofollow">hierarchically porous materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal–organic frameworks (MOFs)&option=203" rel="nofollow">metal–organic frameworks (MOFs);</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nitrogen-doped carbon&option=203" rel="nofollow">nitrogen-doped carbon;</a> </p> <div class="translation"> 机译：CO2减少;电致分析;分层多孔材料;金属有机框架（MOF）;氮掺杂碳; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028161556.html">Highly Efficient Porous Carbon Electrocatalyst with Controllable N‐Species Content for Selective CO2 Reduction</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ye Lin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Ye Lin,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ying Yiran&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Ying Yiran,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Dengrong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Sun Dengrong,</a> <a href="/journal-foreign-19011/" target="_blank" rel="nofollow" class="tuijian_authcolor">Angewandte Chemie .</a> <span>2020</span><span>,第8期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有可控N型含量的高效多孔碳电催化剂，可减少选择性CO2含量</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028355146.html">N-doped hierarchical porous carbon derived from bismuth salts decorated ZIF8 as a highly efficient electrocatalyst for CO2 reduction</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yao Pengfei&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yao Pengfei,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Tianyu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Li Tianyu,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Qiu Yanling&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Qiu Yanling,</a> <a href="/journal-foreign-35176/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Materials Chemistry, A. 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