...
首页> 外文期刊>Progress in Artificial Intelligence >Broadband perovskite quantum dot spectrometer beyond human visual resolution
【24h】

Broadband perovskite quantum dot spectrometer beyond human visual resolution

机译:宽带Perovskite量子点光谱仪超出人类视觉分辨率

获取原文
获取原文并翻译 | 示例
           

摘要

The quantum dot spectrometer, fabricated by integrating different quantum dots with an image sensor to reconstruct the target spectrum from spectral-coupled measurements, is an emerging and promising hyperspectrometry technology with high resolution and a compact size. The spectral resolution and spectral range of quantum dot spectrometers have been limited by the spectral variety of the available quantum dots and the robustness of algorithmic reconstruction. Moreover, the spectrometer integration of quantum dots also suffers from inherent photoluminescence emission and poor batch-to-batch repeatability. In this work, we developed nonemissive in situ fabricated MA(3)Bi(2)X(9) and Cs2SnX6 (MA = CH3NH3; X = Cl, Br, I) perovskite-quantum-dot-embedded films (PQDFs) with precisely tunable transmittance spectra for quantum dot spectrometer applications. The resulting PQDFs contain in situ fabricated perovskite nanocrystals with homogenous dispersion in a polymeric matrix, giving them advantageous features such as high transmittance efficiency and good batch-to-batch repeatability. By integrating a filter array of 361 kinds of PQDFs with a silicon-based photodetector array, we successfully demonstrated the construction of a perovskite quantum dot spectrometer combined with a compressive-sensing-based total-variation optimization algorithm. A spectral resolution of 1.6 nm was achieved in the broadband of 250-1000 nm. The performance of the perovskite quantum dot spectrometer is well beyond that of human eyes in terms of both the spectral range and spectral resolution. This advancement will not only pave the way for using quantum dot spectrometers for practical applications but also significantly impact the development of artificial intelligence products, clinical treatment equipment, scientific instruments, etc.
机译:量子点光谱仪通过将不同的量子点与图像传感器集成来重建从频谱耦合测量的目标光谱,是具有高分辨率和紧凑尺寸的新出现和有前景的高光测量技术。量子点光谱仪的光谱分辨率和频谱范围受到可用量子点的光谱多样的限制以及算法重建的鲁棒性。此外,量子点的光谱仪整合也遭受了固有的光致发光发射和批量间的可重复性。在这项工作中,我们在原位制造的MA(3)BI(2)x(9)和CS2SNX6(MA = CH3NH3; X = CL,BR,I)钙钛矿 - 量子 - 点嵌入薄膜(PQDFS)的不显义用于量子点光谱仪应用的可调透射谱。所得的PQDFS在聚合物基质中含有原位制造的钙钛矿纳米晶体,其在聚合物基质中具有均匀的分散体,使其有利的特征,例如高透射率和良好的批量批量重复性。通过将361种PQDFS的滤波器阵列与基于硅基的光电探测器阵列集成,我们成功地证明了钙钛矿量子点光谱仪的构造,与基于压缩感测的总变化优化算法相结合。在250-1000nm的宽带中实现了1.6nm的光谱分辨率。钙钛矿量子点光谱仪的性能远远超出了人眼的光谱范围和光谱分辨率。这种进步不仅将为实际应用提供量子点光谱仪的方式铺平道路,而且影响人工智能产品,临床治疗设备,科学仪器等显着影响。

著录项

相似文献

  • 外文文献
  • 中文文献
  • 专利
获取原文

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号