Deactivation and Regeneration of NaTaO <sub xmlns='http://www.wiley.com/namespaces/wiley'>3</sub>3 Photocatalyst in Cooperating Dehydrogenation Coupling of Isopropanol and Hydrogenation Coupling of Acetone Reaction System

Cao Baoyue; Yu Yan; Xu Shan; Wang Xiangting; Zhang Li; Wang Zhijian; Wang Shumin; Zhang Guochun

摘要

Abstract > Photocatalyst activity is influenced by many factors, such as adsorption of by‐products, runoff of surface hydroxyl groups and carriers. In this study, a simple and efficient photocatalyst regeneration method was developed. Results indicated that NaTaO <sub>3</sub> photocatalyst lost its photoactivity after three cycles of reaction that involves coupling of isopropanol and hydrogenation coupling of acetone reaction system. Runoff of Na on the surface was the main reason for the deactivation of NaTaO <sub>3</sub> photocatalyst. After hydrothermal treatment of the deactivated NaTaO <sub>3</sub> with 10 <sc>m</sc> Na <fc>OH</fc> at 180°C for 12 h, its photocatalytic activity was restored to the original level. The photocatalytic activity remained stable even after 10 cycles. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：id =“php12856-abs-0001”xml：lang =“en”> <标题类型=“main” >摘要</标题> >光催化剂活性受许多因素的影响，例如副产品的吸附，表面羟基和载体的径流。在这项研究中，开发了一种简单高效的光催化剂再生方法。结果表明，Natao <sub> 3 </ sub>光催化剂在三个反应循环后失去了光度的光度，涉及丙酮反应体系的异丙醇和氢化偶联的偶联。目的上的NA径流是登录Natao <sub> 3 </ sub>光催化剂的主要原因。在180℃下用10-SaON <sub> Na </ she> Na <fc> Na <Fc> Na <Fc> Na <Fc> OH / Fc>在180℃下进行水热处理后12小时，将其光催化活性恢复到原始等级。即使在10个循环之后，光催化活性也保持稳定。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-29317/'>《Photochemistry and Photobiology: An International Journal》</a> <b style="margin: 0 2px;">|</b><span>2018年第3期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Baoyue&option=202" target="_blank" rel="nofollow">Cao Baoyue;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yu Yan&option=202" target="_blank" rel="nofollow">Yu Yan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Shan&option=202" target="_blank" rel="nofollow">Xu Shan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Xiangting&option=202" target="_blank" rel="nofollow">Wang Xiangting;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Li&option=202" target="_blank" rel="nofollow">Zhang Li;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Zhijian&option=202" target="_blank" rel="nofollow">Wang Zhijian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Shumin&option=202" target="_blank" rel="nofollow">Wang Shumin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Guochun&option=202" target="_blank" rel="nofollow">Zhang Guochun;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Shaanxi Key Laboratory of Comprehensive Utilization of Tailings ResourcesShangluo UniversityShangluo China;</p> <p>Shaanxi Key Laboratory of Comprehensive Utilization of Tailings ResourcesShangluo UniversityShangluo China;</p> <p>Shaanxi Key Laboratory of Comprehensive Utilization of Tailings ResourcesShangluo UniversityShangluo China;</p> <p>Shaanxi Key Laboratory of Comprehensive Utilization of Tailings ResourcesShangluo UniversityShangluo China;</p> <p>State Key Laboratory of Coal ConversionChinese Academy of SciencesTaiyuan China;</p> <p>State Key Laboratory of Coal ConversionChinese Academy of SciencesTaiyuan China;</p> <p>Shaanxi Key Laboratory of Comprehensive Utilization of Tailings ResourcesShangluo UniversityShangluo China;</p> <p>Shaanxi Key Laboratory of Comprehensive Utilization of Tailings ResourcesShangluo UniversityShangluo China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/4815.html" title="光化学、辐射化学、超声波作用的化学过程">光化学、辐射化学、超声波作用的化学过程;</a><a href="https://www.zhangqiaokeyan.com/clc/1345.html" title="生物光学">生物光学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> </p> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704024468267.html">Deactivation and Regeneration of NaTaO <sub xmlns="http://www.wiley.com/namespaces/wiley">3</sub>3 Photocatalyst in Cooperating Dehydrogenation Coupling of Isopropanol and Hydrogenation Coupling of Acetone Reaction System</a> <b>[J]</b> . <span> <a 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Deactivation and Regeneration of NaTaO 33 Photocatalyst in Cooperating Dehydrogenation Coupling of Isopropanol and Hydrogenation Coupling of Acetone Reaction System

摘要

Deactivation and Regeneration of NaTaO ₃3 Photocatalyst in Cooperating Dehydrogenation Coupling of Isopropanol and Hydrogenation Coupling of Acetone Reaction System