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Active Sites Intercalated Ultrathin Carbon Sheath on Nanowire Arrays as Integrated Core–Shell Architecture: Highly Efficient and Durable Electrocatalysts for Overall Water Splitting

机译：活性位点在纳米线阵列上插入超薄碳护套作为集成的核心壳结构：用于整体水分裂的高效和耐用的电催化剂

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Abstract > The development of active bifunctional electrocatalysts with low cost and earth‐abundance toward oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) remains a great challenge for overall water splitting. Herein, metallic Ni <sub>4</sub> Mo nanoalloys are firstly implanted on the surface of NiMoO <sub>x</sub> nanowires array (NiMo/NiMoO <sub>x</sub> ) as metal/metal oxides hybrid. Inspired by the superiority of carbon conductivity, an ultrathin nitrogen‐doped carbon sheath intercalated NiMo/NiMoO <sub>x</sub> (NC/NiMo/NiMoO <sub>x</sub> ) nanowires as integrated core–shell architecture are constructed. The integrated NC/NiMo/NiMoO <sub>x</sub> array exhibits an overpotential of 29 mV at 10 mA cm ?2 and a low Tafel slope of 46 mV dec ?1 for HER due to the abundant active sites, fast electron transport, low charge‐transfer resistance, unique architectural structure and synergistic effect of carbon sheath, nanoalloys, and oxides. Moreover, as OER catalysts, the NC/NiMo/NiMoO <sub>x</sub> hybrids require an overpotential of 284 mV at 10 mA cm ?2 . More importantly, the NC/NiMo/NiMoO <sub>x</sub> array as a highly active and stable electrocatalyst approaches ≈10 mA cm ?2 at a voltage of 1.57 V, opening an avenue to the rational design and fabrication of the promising electrode materials with architecture structures toward the electrochemical energy sto </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >开发具有低成本和地球丰富的活性双官能电催化剂对氧气进化反应（OER）和氢进化反应（她）仍然是整个水分裂的巨大挑战。在此，首先植入金属Ni <sub> 4 </ sub> Mo纳米铝在NiMoo Zl和<sub> X / sum> </ i>纳米线阵列的表面上（nimo / nimoo <sub> x </ sub> </ i>）作为金属/金属氧化物杂种。灵感来自碳导电性的优越性，超薄氮掺杂的碳鞘插入Nimo / Nimoo <sub> x </ sub> <sub> x </ sub构建> </ i>）纳米线作为集成核心壳结构。集成的NC / NIMO / NIMOO <I> <亚> x </ sub> </ i>阵列在10 mA cm 2 </ sup>和46 mV的低Tafel斜率下表现出29mV的过电位由于活跃的部位丰富，电子传输，低电荷转移电阻，独特的架构结构和碳鞘，纳米合金和氧化物的协同作用，对她而言，对她而言此外，作为oer催化剂，NC / Nimo / Nimoo <sub> x </ sub> </ i>杂种需要在10 mA cm 2 </ sup>时的过电位为284mV。更重要的是，NC / NIMO / NIMOO <sub> x </ sub> </ i>阵列作为高度活跃且稳定的电催化剂在电压下的≈10macmΔ2</ sup> 1.57 V，对理性设计开放和制造有前途的电极材料，架构结构朝向电化学能量STO </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-28247/'>《Small》</a> <b style="margin: 0 2px;">|</b><span>2017年第46期</span><b style="margin: 0 2px;">|</b><span>共1页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hou Jungang&option=202" target="_blank" rel="nofollow">Hou Jungang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Yunzhen&option=202" target="_blank" rel="nofollow">Wu Yunzhen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Shuyan&option=202" target="_blank" rel="nofollow">Cao Shuyan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Yiqing&option=202" target="_blank" rel="nofollow">Sun Yiqing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Licheng&option=202" target="_blank" rel="nofollow">Sun Licheng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Fine ChemicalsDalian University of Technology (DUT)Dalian 116024 China;</p> <p>State Key Laboratory of Fine ChemicalsDalian University of Technology (DUT)Dalian 116024 China;</p> <p>State Key Laboratory of Fine ChemicalsDalian University of Technology (DUT)Dalian 116024 China;</p> <p>State Key Laboratory of Fine ChemicalsDalian University of Technology (DUT)Dalian 116024 China;</p> <p>State Key Laboratory of Fine ChemicalsDalian University of Technology (DUT)Dalian 116024 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=core–shell architecture&option=203" rel="nofollow">core–shell architecture;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysts&option=203" rel="nofollow">electrocatalysts;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=fast electron transfer&option=203" rel="nofollow">fast electron transfer;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=overall water splitting&option=203" rel="nofollow">overall water splitting;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ultrathin carbon sheath&option=203" rel="nofollow">ultrathin carbon sheath;</a> </p> <div class="translation"> 机译：核心壳结构;电催化剂;快电子转移;总水分裂;超薄碳鞘; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> 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