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Low cost red mud modified graphitic carbon nitride for the removal of organic pollutants in wastewater by the synergistic effect of adsorption and photocatalysis

机译:低成本红泥改性石墨碳氮化物,通过吸附和光催化的协同效应去除废水中的有机污染物

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摘要

The red mud/g-C3N4 (RM-CN) composite was directly prepared via one-step thermal polymerization method using melamine and industrial waste residue (red mud) as raw materials. Under the synergistic effect of adsorption and photocatalysis, RM-CN composites have a significant effect for the removal of organic pollutants from wastewater. Compared with pure CN, the specific surface area of RM-CN has been significantly enhanced with the introduction of RM. Additionality, the optical absorption and photocurrent response exhibit obvious enhancement with respect to RM-CN as compared with that of pristine CN photocatalyst. The optimized 0.8% RM-CN product (with the RM mass content of 0.8 wt% in precursor) displayed referable photocatalytic degradation efficiency for antibiotics and dyes under visible light, as well as excellent recycle performance. This work poses a great potential in the actual wastewater treatment, and it is of great significance to the resource utilization and the cost saving of the raw material.
机译:通过使用三聚氰胺和工业废物残留物(红泥)作为原料,通过一步热聚合方法直接制备红色泥浆/ G-C3N4(RM-CN)复合物。在吸附和光催化的协同作用下,RM-CN复合材料具有显着的效果,用于从废水中除去有机污染物。与纯CN相比,通过引入RM,RM-CN的比表面积显着增强。与原始CN光催化剂相比,相对于RM-CN相对于RM-CN,且光学吸收和光电流响应表现出明显的增强。优化的0.8%RM-CN产品(前体中的RM质量含量为0.8wt%)显示出可见光下的抗生素和染料的可称为光催化降解效率,以及出色的再循环性能。这项工作在实际废水处理中造成了巨大的潜力,对资源利用率和原料的成本节省具有重要意义。

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