Superamphiphobic Coatings from Combination of a Biomimetic Catechol‐Bearing Fluoropolymer and Halloysite Nanotubes

Ma Wei; Higaki Yuji; Takahara Atsushi

摘要

Abstract > Superamphiphobic coatings with remarkable water and oil repellency are prepared by the combination of a biomimetic catechol‐bearing fluoropolymer, poly{2‐(perfluorooctyl)ethyl acrylate‐ co ‐ N ‐(3,4‐dihydroxyphenethyl) acrylamide} (P(FAC <sub>8</sub> ‐ co ‐DOPAm)), and naturally available halloysite nanotubes (HNTs). They are based on surface modification of HNTs with P(FAC <sub>8</sub> ‐ co ‐DOPAm). A procedure to attain stable affinity between silica and the copolymer is established, and used for surface modification of HNTs. Superamphiphobic coatings are obtained by casting the suspension of P(FAC <sub>8</sub> ‐ co ‐DOPAm)‐modified HNTs onto substrates. The superamphiphobic coatings exhibit Cassie–Baxter's wetting to liquids with a wide range of surface tension, because of the extremely low surface free energy and the unique micro‐/nanohierarchical surface topography, as well as the re‐entrant curvature of HNTs. These superamphiphobic coatings are environmentally and chemically durable, and can resist water scouring. The abundance of HNTs in nature and the easily controlled process of this method ensure an efficient approach for large‐scale production of superamphiphobic coatings for various applications. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 具有显着水和防油脂的超人物涂层通过仿生儿茶酚含氟聚合物，聚{2-（全氟胶辛基）乙基丙烯酸酯 - co </ i> - n </ i> - （3,4-二羟基乙基）丙烯酰胺}（P（FAC <sub> 8 </ sub> - co </ i> -Dopam）），天然可用的Holloysite Nanotubes（HNT）。它们基于具有P的HNT的表面改性（FAC <sub> 8 </ sub> - co </ i> -dopam）。建立在二氧化硅和共聚物之间获得稳定亲和力的方法，并用于HNT的表面改性。 Superamphiphiphic涂层是通过铸造P的悬浮液而获得的（FAC <sub> 8 </ sub> - co </ i> -dopam） - 在基板上进行处理。超人物涂层表现出Cassie-Baxter对液体润湿，具有宽范围的表面张力，因为极低的表面自由能和独特的微/纳米级表面形貌，以及HNT的再参赛体曲率。这些超级白斑涂层环境和化学耐用，可以抵抗水冲洗。本质上的HNT的丰度和该方法的易受控制过程确保了用于各种应用的大规模生产的高尺寸生产方法。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第23期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ma Wei&option=202" target="_blank" rel="nofollow">Ma Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Higaki Yuji&option=202" target="_blank" rel="nofollow">Higaki Yuji;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Takahara Atsushi&option=202" target="_blank" rel="nofollow">Takahara Atsushi;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Institute for Materials Chemistry and EngineeringKyushu University744 Motooka Fukuoka 819‐0395 Japan;</p> <p>Institute for Materials Chemistry and EngineeringKyushu University744 Motooka Fukuoka 819‐0395 Japan;</p> <p>Institute for Materials Chemistry and EngineeringKyushu University744 Motooka Fukuoka 819‐0395 Japan;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=catechol&option=203" rel="nofollow">catechol;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=halloysite&option=203" rel="nofollow">halloysite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanotube&option=203" rel="nofollow">nanotube;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=superamphiphobic&option=203" rel="nofollow">superamphiphobic;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=superoleophobic&option=203" rel="nofollow">superoleophobic;</a> </p> <div class="translation"> 机译：儿茶酚;哈利亚特;纳米管;超人物;超级药物; 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