3D Highly Conductive Silver Nanowire@PEDOT:PSS Composite Sponges for Flexible Conductors and Their All‐Solid‐State Supercapacitor Applications

Moon In Kyu; Yoon Seonno; Oh Jungwoo

摘要

Abstract > Although increasing attention has been paid to wearable electronic devices in recent years, flexible supercapacitors with high performance remain not readily available because of the limitations of flexible electrode types. A highly conductive 3D macroporous sponge is fabricated by coating poly(3,4‐ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS)/silver nanowires (AgNWs) on a commercial sponge using a simple and low‐cost “immersion method.” The fabricated flexible 3D sponge conductor shows a high electrical conductivity of 3.94 × 10 ?4 S cm ?1 with good stability in various environments and under bending deformation. To exploit the potential of the flexible 3D PEDOT:PSS/AgNW coating on the sponge as a current collector for energy‐related applications, urchin‐like Co(OH)F arrays are directly grown on PEDOT:PSS/AgNW‐on‐sponge conductors for all‐solid‐state supercapacitors. The resulting symmetric all‐solid‐state supercapacitor exhibits a mass‐specific capacitance of 103.7 F g ?1 at a current density of 1 A g ?1 , retaining 85.8% of the initial capacitance after 3000 cycles, and mechanical flexibility during bending. This fabrication of the 3D lightweight conductor can be easily scaled up for mass production and introduces new opportunities for flexible electronic applications. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 虽然近年来，由于柔性电极类型的局限性，近年来，近年来，越来越高的人的注意力被支付给可穿戴电子设备。使用简单且低成本的“浸入方法”，通过涂布聚（3,4-亚乙二氧基噻吩）：聚（苯乙烯磺酸盐）（PEDOT）（PEDOT：PSS）/银纳米线（AGNWS）来制造高导电3D大孔海绵。制造的柔性3D海绵导体显示出3.94×10的高电导率？4 </ sup> 厘米？1 </ sup> 在各种环境中具有良好的稳定性，并且在弯曲变形下。利用柔性3D转型的潜力：海绵上的PSS / Agnw涂层作为用于能量相关应用的集电器，核苷状CO（OH）F阵列直接在PEDOT上生长：PSS / AgnW-On-Sponge导体适用于全固态超级电容器。得到的对称全固态超级电容器具有103.7f g的质量特异性电容？1 </ sup> 在最小密度为1 a g ？1 </ sup> ，在3000次循环后保留85.8％的初始电容，并在弯曲期间机械柔韧性。这种3D轻质导体的制造可以很容易地扩大批量生产，并为灵活的电子应用引入了新的机会。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第22期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Moon In Kyu&option=202" target="_blank" rel="nofollow">Moon In Kyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yoon Seonno&option=202" target="_blank" rel="nofollow">Yoon Seonno;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Oh Jungwoo&option=202" target="_blank" rel="nofollow">Oh Jungwoo;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Yonsei Institute of Convergence TechnologyYonsei UniversityIncheon 21983 Republic of Korea;</p> <p>Yonsei Institute of Convergence TechnologyYonsei UniversityIncheon 21983 Republic of Korea;</p> <p>Yonsei Institute of Convergence TechnologyYonsei UniversityIncheon 21983 Republic of Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Co(OH)F nanowire arrays&option=203" rel="nofollow">Co(OH)F nanowire arrays;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=flexible conductor&option=203" rel="nofollow">flexible conductor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=PEDOT:PSS&option=203" rel="nofollow">PEDOT:PSS;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=silver nanowire&option=203" rel="nofollow">silver nanowire;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=supercapacitors&option=203" rel="nofollow">supercapacitors;</a> </p> <div class="translation"> 机译：CO（OH）F纳米线阵列;柔性导体;PEDOT：PSS;银纳米线;超级电容器; </div> </li> 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