A Printing‐Centric Approach to the Electrostatic Modification of Polymer/Clay Composites for Use in 3D Direct‐Ink Writing

Rauzan Brittany M.; Lehman Sean E.; McCracken Joselle M.; Lee Jonghun; Lin Xiao‐Min; Sandy Alec; Narayanan Suresh; Rogers Simon A.; Nuzzo Ralph G.

摘要

Abstract > Polymer/clay composite inks are exceptionally useful materials for fabrication processes based on 3D direct‐ink writing, however, there remains an insufficient understanding of how their physiochemical dynamics impact printability. Using a model system, N ‐isopropylacrylamide/Laponite, the electrostatic interactions between Laponite platelets are modified to tune critical rheological properties in order to improve printability. Rheological measurements and X‐ray scattering experiments are carried out to monitor the nano/micro‐structural dynamics and complex physicochemical interactions of Laponite as it impacts complex modulus in the linear region, flow behavior, thixotropy, and yield stress of the composite ink. Modification of the electrostatic interactions between platelets reduces the yield stress of the material, while maintaining a complex microstructure that allows for sufficient recovery times upon removal of stress to form stable, and thus printable, filaments. A printing‐centric approach is established based on a fundamental understanding of electrostatic inter‐particle interactions, harnessing the innate microstructure of Laponite in 3D direct‐ink writing of composites. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 聚合物/粘土复合墨水是基于3D直接墨水写入的制造过程的特殊用材料，但是，对其物理动力学如何影响可印刷性的影响仍然不足。使用模型系统， n </ i> - 丙基丙烯酰胺/氯尼钛矿，氯代岩血小板之间的静电相互作用被修饰以调节临界流变性能，以提高可印刷性。进行流变测量和X射线散射实验，以监测纳隆岩的纳米/微结构动力学和复杂的物理化学相互作用，因为它会影响线性区域，流动性，触变性和屈服应力的复合模量影响复合油墨的屈服应力。血小板之间的静电相互作用的改变降低了材料的屈服应力，同时保持复杂的微观结构，其在去除应力后允许足够的恢复时间形成稳定，因此可打印，长丝。基于对静电颗粒相互作用的基本理解建立了一种印刷的方法，利用了三维直接墨水写入复合材料中的Laponite的先天微观结构。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces 》</a> <b style="margin: 0 2px;">|</b><span>2018年第8期</span><b style="margin: 0 2px;">|</b> <span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Rauzan Brittany M.&option=202" target="_blank" rel="nofollow">Rauzan Brittany M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lehman Sean E.&option=202" target="_blank" rel="nofollow">Lehman Sean E.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=McCracken Joselle M.&option=202" target="_blank" rel="nofollow">McCracken Joselle M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Jonghun&option=202" target="_blank" rel="nofollow">Lee Jonghun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Xiao‐Min&option=202" target="_blank" rel="nofollow">Lin Xiao‐Min;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sandy Alec&option=202" target="_blank" rel="nofollow">Sandy Alec;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Narayanan Suresh&option=202" target="_blank" rel="nofollow">Narayanan Suresh;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Rogers Simon A.&option=202" target="_blank" rel="nofollow">Rogers Simon A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nuzzo Ralph G.&option=202" target="_blank" rel="nofollow">Nuzzo Ralph G.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of ChemistryUniversity of Illinois at Urbana‐Champaign600 S. Matthews Avenue Urbana IL 61801 USA;</p> <p>Department of ChemistryUniversity of Illinois at Urbana‐Champaign600 S. Matthews Avenue Urbana IL 61801 USA;</p> <p>Department of ChemistryUniversity of Illinois at Urbana‐Champaign600 S. Matthews Avenue Urbana IL 61801 USA;</p> <p>X‐ray Science DivisionArgonne National Laboratory9700 South Cass Avenue Argonne IL 60439 USA;</p> <p>Center for Nanoscale MaterialsArgonne National Laboratory9700 South Cass Avenue Argonne IL 60439 USA;</p> <p>X‐ray Science DivisionArgonne National Laboratory9700 South Cass Avenue Argonne IL 60439 USA;</p> <p>X‐ray Science DivisionArgonne National Laboratory9700 South Cass Avenue Argonne IL 60439 USA;</p> <p>Department of Chemical and Biomolecular EngineeringUniversity of Illinois at Urbana‐Champaign600 S. Matthews Avenue Urbana IL 61801 USA;</p> <p>Department of ChemistryUniversity of Illinois at Urbana‐Champaign600 S. Matthews Avenue Urbana IL 61801 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=direct‐ink write&option=203" rel="nofollow">direct‐ink write;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogels&option=203" rel="nofollow">hydrogels;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanocomposites&option=203" rel="nofollow">nanocomposites;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polymers&option=203" rel="nofollow">polymers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=rheo‐SAXS&option=203" rel="nofollow">rheo‐SAXS;</a> </p> <div class="translation"> 机译：直接墨水写;水凝胶;纳米复合材料;聚合物;Rheo-SAXS; 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=姜爱峰&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,姜爱峰</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘钢&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,刘钢</a> <span> <a href="/conference-cn-61775/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2017年江苏科技论坛绿色公路分论坛暨公路养护技术国际学术会议 </a> <span> <span> . 2017</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/02031652048.html">聚合物/改性粘土纳米复合材料的新型合成方法和性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=宋磊&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 宋磊</a> <span> . 2002</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061202756272.html">一种新型粘土改性方法及利用该粘土制备聚合物复合材料的方法</a> <b>[P]</b> . <span> 中国专利： CN105885022B </span> <span> . 2018.01.30</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120108370932.html">一种新型粘土改性方法及利用该粘土制备聚合物复合材料的方法</a> <b>[P]</b> . <span> 中国专利： CN105885022A </span> <span> . 2016-08-24</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130444672281.html">Process for preparing an aqueous polymer dispersion nanocompu00f3sita clay dispersion aqueous nanocompu00f3sita, thickener, dispersant, binder, the composition of the flexographic ink.On Printing varnish, modifier of cement powder dry, seed nanocompu00f3sita polymer clay, polymer composition nanocompu00f3sita of clay, and,Method for preparing a plurality of partu00ecculas clay hollow polymeric nanocompu00f3sitas</a> <b>[P]</b> . <span> 外国专利：  BR0113999A </span> <span> . 2003-08-12</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：水性聚合物分散体纳米复合材料的制备方法水性粘土纳米分散体，增稠剂，分散剂，粘合剂，柔性版印刷油墨的组成。在印刷清漆上，水泥干粉的改性剂，种子纳米复合材料，聚合物纳米复合材料粘土，以及制备多部分粘土空心聚合物纳米复合材料的方法 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130424533054.html">MANUFACTURING METHOD AND AN OMNIDIRECTIONAL WRITING METHOD OF A 3D CONDUCTING POLYMER ULTRAFINE WIRE, AND THE 3D CONDUCTING POLYMER ULTRAFINE WIRE AND WRITING OBTAINED BY THE SAME</a> <b>[P]</b> . <span> 外国专利：  KR20110086253A </span> <span> . 2011-07-28</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：3D导电聚合物超细电线的制造方法和单向写入方法，以及获得的3D导电聚合物超细电线的相同制造方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130424432911.html">Manufacturing method and omnidirectional writing method of a 3D conducting polymer ultrafine wire, and 3D conducting polymer ultrafine wire and writing obtained by the same</a> <b>[P]</b> . <span> 外国专利：  KR101069587B1 </span> <span> . 2011-10-05</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：3d导电聚合物超细导线的制造方法和全向写入方法以及3d导电聚合物超细导线和由此获得的写入 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022435622','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div 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