Macroscopic‐Oriented Gold Nanorods in Polyvinyl Alcohol Films for Polarization‐Dependent Multicolor Displays

Dai Liwei; Lu Xuefei; Song Liping; Huang Youju; Liu Baoqing; Zhang Lei; Zhang Jiawei; Wu Si; Chen Tao

摘要

Abstract >Due to their abundant optical colors, durable color generation, and high refreshing rate, smart chromic nanomaterials (SCNMs) have been employed in various applications. However, most SCNMs often require multicomponent materials, precise morphology control, and complicated modulation to realize multicolor changes, which limits their widely practical applications. In the present study, a simple and effective strategy is demonstrated to achieve the flexible and cost‐effective multicolor gold nanorods (Au NRs)/polymer hybrid film, by tuning macroscopic‐oriented Au NRs in films and a synergy of polarization‐dependent surface plasmon resonance. Au NRs are first functionalized with methoxypoly(ethylene glycol)thiol to improve the compatibility, ensuring Au NRs can be homogenously dispersed in the polyvinyl alcohol (PVA) matrix with high particle density. The macroscopic‐oriented alignment of Au NRs can be achieved by the elongation of the PVA polymer molecular chains. Under different polarized excitation directions, the same strip of the hybrid film exhibits various colors including red, orange, yellow, and green. Therefore, the strategy provides a simple and powerful approach to achieve macroscopic‐oriented anisotropic nanoparticles in the polymer matrix, and the resultant hybrid films are promising in various practical applications, such as color displays, optical devices, and plasmonic biosensors. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >由于它们丰富的光学颜色，耐用的颜色和高刷新率，智能铬纳米材料（SCNMS）已经采用了各种应用。然而，大多数SCNMS通常需要多组分材料，精确的形态控制和复杂的调制来实现多色变化，这限制了它们广泛的实际应用。在本研究中，通过调整薄膜中的宏观导向的Au NRS来实现简单且有效的策略，以实现柔性且经济高效的多色金纳米棒（Au NRS）/聚合物杂化膜，以及偏振依赖性表面等离子体的协同作用谐振。 Au NRS首先用甲氧基聚（乙二醇）硫醇官能化以改善相容性，确保Au NR可以以高粒子密度均匀地分散在聚乙烯醇（PVA）基质中。通过PVA聚合物分子链的伸长可以实现Au NRS的宏观取向。在不同的极化激发方向下，相同的混合膜条具有各种颜色，包括红色，橙色，黄色和绿色。因此，该策略提供了一种简单且强大的方法来实现聚合物基质中的宏观导向的各向异性纳米颗粒，并且所得的杂种膜在各种实际应用中具有很大的意识，例如彩色显示器，光学装置和等离子体化学体。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces 》</a> <b style="margin: 0 2px;">|</b><span>2018年第11期</span><b style="margin: 0 2px;">|</b> <span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dai Liwei&option=202" target="_blank" rel="nofollow">Dai Liwei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lu Xuefei&option=202" target="_blank" rel="nofollow">Lu Xuefei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Song Liping&option=202" target="_blank" rel="nofollow">Song Liping;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Youju&option=202" target="_blank" rel="nofollow">Huang Youju;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Baoqing&option=202" target="_blank" rel="nofollow">Liu Baoqing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Lei&option=202" target="_blank" rel="nofollow">Zhang Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Jiawei&option=202" target="_blank" rel="nofollow">Zhang Jiawei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Si&option=202" target="_blank" rel="nofollow">Wu Si;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Tao&option=202" target="_blank" rel="nofollow">Chen Tao;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> <p>Max Planck Institute for Polymer ResearchAckermannweg 10 Mainz D‐55128 Germany;</p> <p>Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=color displays&option=203" rel="nofollow">color displays;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=gold nanorods&option=203" rel="nofollow">gold nanorods;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=macroscopic alignment&option=203" rel="nofollow">macroscopic alignment;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oriented&option=203" rel="nofollow">oriented;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polarization&option=203" rel="nofollow">polarization;</a> </p> <div class="translation"> 机译：彩色显示;金纳米棒;宏观对齐;定向;极化; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022435387.html">Macroscopic‐Oriented Gold Nanorods in Polyvinyl Alcohol Films for Polarization‐Dependent Multicolor 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