Apatite Formation on Poly(aryl ether sulfone ketone) Surfaces by Means of Polydopamine Layers Functionalized with Phosphonate Groups

Liu Chengde; Liu Cheng; Gao Yu; Cheng Fang; Xiao Gary G.; Wang Jinyan; Jian Xigao

摘要

Abstract > Poly(aryl ether sulfone ketone) containing phthalazinone and biphenyl moieties (PPBESK) is a promising candidate for replacing metal bone implants. Apatite synthesized by polydopamine‐assisted hydroxyapatite formation (pHAF) is a promising coating for bone‐implant application. In this study, a modified pHAF technique is employed to induce the formation of apatite onto PPBESK while phosphonate groups, as potent inducers of apatite formation, are introduced through modification of a polydopamine (PDA) layer. The PPBESK layer and surface‐modified samples are evaluated by Raman spectroscopy, contact angle measurement, scanning electron microscope (SEM), and X‐ray photoelectron spectroscopy, respectively. The surface roughness of the samples increases following self‐polymerization of dopamine and decreases after reacting with POCl <sub>3</sub> . PPBESK water contact angle reduces significantly after coating with PDA. Microstructural and compositional analyses by SEM and X‐ray diffraction reveal that apatite coating induced by phosphonate groups exhibits a greater quantity of apatite formation, a higher ratio of Ca/P than that induced by a pristine PDA layer. The surfaces are characterized by culturing with MC3T3‐E1 preosteoblasts. Apatite induced by phosphonate group conjugated to PDA layer on PPBESK surface promotes cytocompatibility and osteogenesis of MC3T3‐E1 preosteoblasts in vitro. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 含有酞嗪酮和联苯基部分（PPBESK）的聚（芳基醚砜酮）是用于更换金属骨植入物的有望候选者。通过聚二胺辅助羟基磷灰石形成（PHAF）合成的磷灰石是骨植入施用的有希望的涂层。在该研究中，使用改性的PHAF技术将磷灰石的形成诱导在PPBESK上，而膦酸盐基团作为磷灰石形成有效诱导剂，通过改性聚德多样（PDA）层。通过拉曼光谱，接触角测量，扫描电子显微镜（SEM）和X射线光电子能谱评估PPBESK层和表面改性样品。样品的表面粗糙度随着多巴胺的自聚聚，并在与POCl反应后降低 <sub> 3 </ sub> 。 PPBESK与PDA涂层后，水接触角度显着减少。 SEM和X射线衍射的微观结构和组成分析表明，膦酸盐基团诱导的磷灰石涂层表现出更大量的磷灰石形成，Ca / p比由原始PDA层诱导的较高比例。该表面的特征在于用MC3T3-E1培养蛋白细胞培养。通过在PPBESK表面上缀合至PDA层的膦酸盐基团诱导的磷灰石促进了体外MC3T3-E1预卵细胞的细胞相容性和骨质发生。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第13期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Chengde&option=202" target="_blank" rel="nofollow">Liu Chengde;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Cheng&option=202" target="_blank" rel="nofollow">Liu Cheng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gao Yu&option=202" target="_blank" rel="nofollow">Gao Yu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cheng Fang&option=202" target="_blank" rel="nofollow">Cheng Fang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xiao Gary G.&option=202" target="_blank" rel="nofollow">Xiao Gary G.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Jinyan&option=202" target="_blank" rel="nofollow">Wang Jinyan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jian Xigao&option=202" target="_blank" rel="nofollow">Jian Xigao;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Fine ChemicalsDalian University of TechnologyDalian 116024 China;</p> <p>State Key Laboratory of Fine ChemicalsDalian University of TechnologyDalian 116024 China;</p> <p>Department of Polymer Science &</p> <p>EngineeringDalian University of TechnologyDalian 116024 China;</p> <p>State Key Laboratory of Fine ChemicalsDalian University of TechnologyDalian 116024 China;</p> <p>School of Pharmaceutical Science and TechnologyDalian University of TechnologyDalian 116024 China;</p> <p>Department of Polymer Science &</p> <p>EngineeringDalian University of TechnologyDalian 116024 China;</p> <p>Department of Polymer Science &</p> <p>EngineeringDalian University of TechnologyDalian 116024 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=apatite coatings&option=203" rel="nofollow">apatite coatings;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=phosphonate groups&option=203" rel="nofollow">phosphonate groups;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=poly(aryl ether sulfone ketone)&option=203" rel="nofollow">poly(aryl ether sulfone ketone);</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polydopamine&option=203" rel="nofollow">polydopamine;</a> </p> <div class="translation"> 机译：磷灰石涂层;膦酸盐基团;聚（芳基醚砜酮）;聚二胺; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434755.html">Apatite Formation on Poly(aryl ether sulfone ketone) Surfaces by Means of Polydopamine Layers Functionalized with Phosphonate Groups</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Chengde&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Liu Chengde,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Cheng&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Liu Cheng,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gao Yu&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Gao Yu,</a> <a href="/journal-foreign-18063/" target="_blank" rel="nofollow" class="tuijian_authcolor">Advanced materials interfaces .</a> <span>2018</span><span>,第13期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：通过用膦酸酯基团官能化的聚二胺层对聚（芳基醚砜酮酮）表面形成磷灰石形成</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_macromolecular-chemistry-physics_thesis/020418430111.html">A novel synthesis and characterization of phenylacetylene end-capped poly(aryl ether sulfone) and poly(aryl ether ketone) oligomers</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mathew Kozuch&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Mathew Kozuch,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Angela Schaffer&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Angela Schaffer,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Atul Bhatnagar&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Atul Bhatnagar,</a> <a href="/journal-foreign-13602/" target="_blank" rel="nofollow" class="tuijian_authcolor">Macromolecular chemistry and physics .</a> <span>1995</span><span>,第7期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：苯乙炔封端的聚（芳基醚砜）和聚（芳基醚酮）低聚物的新颖合成和表征</span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/07040599005.html">Naphthalene-based poly(aryl ether)s. .1. 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2005</span><span>,第3期</span> </span> </div> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/academic-journal-cn_journal-jiangxi-normal-university-natural-science-edition_thesis/0201297157445.html">亲电聚合路线合成聚芳醚酮的研究——聚醚醚酮酮砜的合成及表征</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=蔡明中&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 蔡明中</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=宋才生&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,宋才生</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=周丽云&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,周丽云</a> <span> <a href="/journal-cn-50313/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 江西师范大学学报：自然科学版 </a> </span> <span> . 1993</span><span>,第1期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_detail_thesis/0201296398301.html">磺化聚芳醚酮砜中磺酸基团的降解动力学</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王哲&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 王哲</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨鑫&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,杨鑫</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=倪宏哲&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,倪宏哲</a> <span> <a href="/journal-cn-56862/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 高分子材料科学与工程 </a> </span> <span> . 2011</span><span>,第5期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-20216_thesis/0202251367.html">双邻位甲基取代聚芳醚酮酮醚酮酮/聚芳醚醚酮酮无规共聚物的合成与表征</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=夏俊&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 夏俊</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=江西师范大学化学化工学院&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,江西师范大学化学化工学院</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘勇军&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,刘勇军</a> <span> <a href="/conference-cn-20216/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2007年全国塑料改性及合金工业技术交流年会 </a> <span> <span> . 2007</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020313231654.html">含2，6--萘、联苯结构的聚芳醚酮砜及含1，4--萘结构的聚芳醚酮的合成及性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=周文祥&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 周文祥</a> <span> . 2014</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120103970064.html">包含聚(芳基醚砜)、聚(芳基醚酮)、至少一种聚苯硫醚以及玻璃纤维的玻璃填充的聚合物组合物</a> <b>[P]</b> . <span> 中国专利： CN111032783A </span> <span> . 2020-04-17</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120113499154.html">一种聚（芳基醚酮）的制备方法及聚（芳基醚酮）</a> <b>[P]</b> . <span> 中国专利： CN113527661A </span> <span> . 2021-10-22</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130419097886.html">Cement composition, useful for cementing tube well penetrating underground formation by compression, comprises e.g. material including poly (aryl ether ketone) consisting of e.g. polyetheretherketone and poly (biphenyl ether sulfone)</a> <b>[P]</b> . <span> 外国专利：  FR2979911A1 </span> <span> . 2013-03-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：水泥组合物可用于通过压缩使水泥井管很好地渗透到地下地层中，包括例如水泥。包括聚（芳基醚酮）的材料，例如由聚醚醚酮和聚（联苯醚砜） </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130409942789.html">Gelation, Aerogel Formation and Reactions Thereof to Produce Non-Random Functionalization of Poly (Aryl Ether Ketones)</a> <b>[P]</b> . <span> 外国专利：  US2017253712A1 </span> <span> . 2017-09-07</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：凝胶化，气凝胶形成及其反应以产生聚芳醚酮的非随机官能化 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130411735703.html">GELATION, AEROGEL FORMATION AND REACTIONS THEREOF TO PRODUCE NON-RANDOM FUNCTIONALIZATION OF POLY (ARYL ETHER KETONES)</a> <b>[P]</b> . <span> 外国专利：  WO2016040293A1 </span> <span> . 2016-03-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：凝胶化，气凝胶形成及其反应，以产生聚（芳族醚酮）的非随机功能 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022434755','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p 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