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Unlocking the Single‐Domain Epitaxy of Halide Perovskites

机译：解锁卤化物植物的单个域外延

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Abstract >The growth of epitaxial semiconductors and oxides has long since revolutionized the electronics and optics fields, and continues to be exploited to uncover new physics stemming from quantum interactions. While the recent emergence of halide perovskites offers exciting new opportunities for a range of thin‐film electronics, the principles of epitaxy have yet to be applied to this new class of materials and the full potential of these materials is still not yet known. In this work, single‐domain inorganic halide perovskite epitaxy is demonstrated. This is enabled by reactive vapor phase deposition onto single crystal metal halide substrates with congruent ionic interactions. For the archetypical halide perovskite, cesium tin bromide, two epitaxial phases, a cubic phase and tetragonal phase, are uncovered which emerge via stoichiometry control that are both stabilized with vastly differing lattice constants and accommodated via epitaxial rotation. This epitaxial growth is exploited to demonstrate multilayer 2D quantum wells of a halide‐perovskite system. This work ultimately unlocks new routes to push halide perovskites to their full potential. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P>外延半导体和氧化物的生长长期以来彻底改变了电子和光学领域，并继续被剥削以发现从量子相互作用的新物理学。虽然最近的卤化物佩罗夫斯基特的出现为一系列薄膜电子产品提供了令​​人兴奋的新机会，但外延的原则尚未适用于这类新的材料，这些材料的全部潜力尚未知道。在这项工作中，证明了单结构域无机卤化物钙钛矿外延。这通过反应性气相沉积在单晶金属卤化物衬底上具有一致离子相互作用的能量。对于原型卤化物钙钛矿，溴化铯，两个外延相，立方相和四方相，其被揭示，其通过化学计量控制出来，所述化学计量控制均稳定，所述晶格常数稳定并通过外延旋转容纳。利用这种外延生长来证明卤化物 - 钙钛矿系统的多层2D量子孔。这项工作最终解锁了新的路线，将卤化物佩罗夫斯克斯推到他们的全部潜力。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第22期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Lili&option=202" target="_blank" rel="nofollow">Wang Lili;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Pei&option=202" target="_blank" rel="nofollow">Chen Pei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Thongprong Non&option=202" target="_blank" rel="nofollow">Thongprong Non;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Young Margaret&option=202" target="_blank" rel="nofollow">Young Margaret;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kuttipillai Padmanaban S.&option=202" target="_blank" rel="nofollow">Kuttipillai Padmanaban S.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Chuanpeng&option=202" target="_blank" rel="nofollow">Jiang Chuanpeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Pengpeng&option=202" target="_blank" rel="nofollow">Zhang Pengpeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Kai&option=202" target="_blank" rel="nofollow">Sun Kai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Duxbury Phillip M.&option=202" target="_blank" rel="nofollow">Duxbury Phillip M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lunt Richard R.&option=202" target="_blank" rel="nofollow">Lunt Richard R.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical Engineering and Materials ScienceMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Chemical Engineering and Materials ScienceMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Physics and AstronomyMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Chemical Engineering and Materials ScienceMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Chemical Engineering and Materials ScienceMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Physics and AstronomyMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Physics and AstronomyMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Material Science and EngineeringUniversity of MichiganAnn Arbor MI 48109 USA;</p> <p>Department of Physics and AstronomyMichigan State UniversityEast Lansing MI 48824 USA;</p> <p>Department of Chemical Engineering and Materials ScienceMichigan State UniversityEast Lansing MI 48824 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=2D quantum well&option=203" rel="nofollow">2D quantum well;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=epitaxy&option=203" rel="nofollow">epitaxy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=halide perovskites&option=203" rel="nofollow">halide perovskites;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=single‐domain&option=203" rel="nofollow">single‐domain;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=vapor‐deposition&option=203" rel="nofollow">vapor‐deposition;</a> </p> <div class="translation"> 机译：2D量子阱;外延;卤化物蠕动;单域;气相沉积; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022435900.html">Perovskites: Unlocking the Single‐Domain Epitaxy of Halide Perovskites (Adv. 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Interfaces 22/2017)</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Lili&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Wang Lili,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Pei&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Chen Pei,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Thongprong Non&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Thongprong Non,</a> <a href="/journal-foreign-18063/" target="_blank" rel="nofollow" class="tuijian_authcolor">Advanced materials interfaces .</a> <span>2017</span><span>,第22期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：Perovskites：解锁卤化物佩罗夫斯基斯的单域外延（ADV。母体。界面22/2017）</span> </p> </li> <li> <div> <b>2. </b><a 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