Atomic Layer Deposited TiO        <sub >2</sub>2        –IrO        <i >          <sub>x</sub>                  <sub >x</sub>x                Alloy as a Hole Transport Material for Perovskite Solar Cells

Tan Wanliang; Hendricks Olivia L.; Meng Andrew C.; Braun Michael R.; McGehee Michael D.; Chidsey Christopher E. D.; McIntyre Paul C.

摘要

Abstract > The hole transport layer (HTL) is one of the key components in planar perovskite solar cells. This study reports a new kind of HTL fabricated using atomic layer deposition (ALD). By alloying TiO <sub>2</sub> with IrO <sub>x</sub> , it is demonstrated that TiO <sub>2</sub> , a well‐known electron‐selective contact and electron transport layer in photovoltaic devices, can behave as an HTL with an appropriately high work function. Perovskite Cs <sub>0.17</sub> FA <sub>0.83</sub> Pb(I <sub>0.83</sub> Br <sub>0.17</sub> ) <sub>3</sub> solar cells including this new hole transport material achieve a power conversion efficiency of 15.8% under AM?1.5G simulated solar irradiation compared to a 14.3% efficiency for otherwise‐identical devices incorporating a more standard NiO HTL layer. These results suggest the promise of transition metal oxide alloys synthesized by ALD as hole contact materials for optoelectronic devices, including advanced photovoltaics. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 空穴传输层（HTL）是平面Perovskite太阳能电池中的关键部件之一。本研究报告了使用原子层沉积（ALD）制造的新种类HTL。通过合金化的TiO. <sub> 2 </ sub> 用伊罗 <sub> x </ sub> </ i> ，据证明TiO <sub> 2 </ sub> ，在光伏器件中众所周知的电子选择性接触和电子传输层，可以表现为具有适当高功函数的HTL。 Perovskite CS. <sub> 0.17 </ sub> F A <sub> 0.83 </ sub> PB（I. <sub> 0.83 </ sub> 布鲁斯 <sub> 0.17 </ sub> 的） <sub> 3 </ sub> 包括该新孔输送材料的太阳能电池在AMα1.5g模拟太阳辐射下实现15.8％的电力转换效率，而另外相同的装置的效率为14.3％，则包含更标准的NiO HTL层。这些结果表明由ALD作为光电器件的孔接触材料合成的过渡金属氧化物合金的承诺，包括高级光伏。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第16期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tan Wanliang&option=202" target="_blank" rel="nofollow">Tan Wanliang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hendricks Olivia L.&option=202" target="_blank" rel="nofollow">Hendricks Olivia L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Meng Andrew C.&option=202" target="_blank" rel="nofollow">Meng Andrew C.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Braun Michael R.&option=202" target="_blank" rel="nofollow">Braun Michael R.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=McGehee Michael D.&option=202" target="_blank" rel="nofollow">McGehee Michael D.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chidsey Christopher E. D.&option=202" target="_blank" rel="nofollow">Chidsey Christopher E. D.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=McIntyre Paul C.&option=202" target="_blank" rel="nofollow">McIntyre Paul C.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Materials Science and EngineeringStanford UniversityStanford CA 94305 USA;</p> <p>Department of ChemistryStanford UniversityStanford CA 94305 USA;</p> <p>Department of Materials Science and EngineeringStanford UniversityStanford CA 94305 USA;</p> <p>Department of Materials Science and EngineeringStanford UniversityStanford CA 94305 USA;</p> <p>Department of Materials Science and EngineeringStanford UniversityStanford CA 94305 USA;</p> <p>Department of ChemistryStanford UniversityStanford CA 94305 USA;</p> <p>Department of Materials Science and EngineeringStanford UniversityStanford CA 94305 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=atomic layer deposition&option=203" rel="nofollow">atomic layer deposition;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=alloy&option=203" rel="nofollow">alloy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hole transport materials&option=203" rel="nofollow">hole transport materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=perovskite solar cells&option=203" rel="nofollow">perovskite solar cells;</a> </p> <div class="translation"> 机译：原子层沉积;合金;孔运输材料;钙钛矿太阳能电池; 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href="/academic-conference-cn_meeting-3189_thesis/02022731193.html">原子层沉积AlOx对无空穴传输材料钙钛矿太阳能电池性能影响研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=卫会云&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 卫会云</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=石将建&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,石将建</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=许信&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,许信</a> <span> <a href="/conference-cn-3189/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第一届新型太阳能电池暨钙钛矿太阳能电池学术研讨会 </a> <span> <span> . 2014</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020312444780.html">基于高效TiO2支架层的无空穴传输层碳基钙钛矿太阳能电池研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=肖雨晴&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 肖雨晴</a> <span> . 2019</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120109855937.html">用于汽车钙钛矿太阳能电池的空穴传输材料、包括其的钙钛矿太阳能电池及其制造方法</a> <b>[P]</b> . <span> 中国专利： CN107359245A </span> <span> . 2017-11-17</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061202838575.html">空穴传输材料及包含该材料的钙钛矿太阳能电池的制备方法</a> <b>[P]</b> . <span> 中国专利： CN105789454B </span> <span> . 2018.05.01</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130400624482.html">HOLE-TRANSPORT MATERIALS FOR PEROVSKITE SOLAR CELL AND THE MANUFACTURING METHOD THEREOF AND THE PEROVSKITE SOLAR CELL COMPRISING THE HOLE-TRANSPORT MATERIALS</a> <b>[P]</b> . <span> 外国专利：  KR102104046B1 </span> <span> . 2020-04-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：钙钛矿太阳能电池的孔穴运输材料及其制造方法和包括该孔穴运输材料的钙钛矿太阳能电池 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130403289488.html">HOLE-TRANSPORT MATERIALS FOR PEROVSKITE SOLAR CELL AND THE MANUFACTURING METHOD THEREOF AND THE PEROVSKITE SOLAR CELL COMPRISING THE HOLE-TRANSPORT MATERIALS</a> <b>[P]</b> . <span> 外国专利：  KR20190050625A </span> <span> . 2019-05-13</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：钙钛矿太阳能电池的孔穴运输材料及其制造方法和包括该孔穴运输材料的钙钛矿太阳能电池 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130408653294.html">A HOLE TRANSPORTING MATERIAL HAVING HIGH HEAT-RESISTING PROPERTY A PEROVSKITE SOLAR CELL COMPRISING THE SAME AND A METHOD OF MANUFACTURING THE PEROVSKITE SOLAR CELL</a> <b>[P]</b> . <span> 外国专利：  KR20170114799A </span> <span> . 2017-10-16</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有高耐热性能的孔传输材料包括其的钙钛矿太阳能电池和制造钙钛矿太阳能电池的方法 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022434291','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img 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Atomic Layer Deposited TiO 22 –IrO x xx Alloy as a Hole Transport Material for Perovskite Solar Cells

摘要

Atomic Layer Deposited TiO ₂2 –IrO _x _xx Alloy as a Hole Transport Material for Perovskite Solar Cells