Surface Fluorination of ALD TiO        <sub >2</sub>2        Electron Transport Layer?for Efficient Planar Perovskite Solar Cells

Zardetto Valerio; di Giacomo Francesco; Lifka Herbert; Verheijen Marcel A.; Weijtens Christ H. L.; Black Lachlan E.; Veenstra Sjoerd; Kessels Wilhelmus M. M.; Andriessen Ronn; Creatore Mariadriana

摘要

Abstract > Perovskite solar cells (PSCs) are emerging among the photovoltaic (PV) technologies due to their high power conversion efficiency (PCE) in combination with potentially low cost manufacturing processing. In this contribution, the fabrication of efficient planar n‐i‐p PSCs by the modification of the electron transport layer (ETL) adopted as n‐type contact is demonstrated. Specifically, a fluorine‐based plasma treatment prior to perovskite deposition leads to surface fluorination of the TiO <sub>2</sub> ETL. The presence of fluorine on the TiO <sub>2</sub> surface drastically improves the adhesion between the ALD layer and the methylammonium lead iodide perovskite film, and leads to a more favourable energy band alignment, accompanied by a faster electron carrier extraction at the interface. As consequence of surface fluorination, we observe a significant reduction in the current density‐voltage curve hysteresis with respect to the ALD based reference sample, as well as a remarkable improvement in power conversion efficiency from 4% up to a stable 14.8%. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 由于其高功率转换效率（PCE）与潜在的低成本制造处理，钙钛矿太阳能电池（PSC）在光伏（PV）技术之后出现。在该贡献中，通过通过作为n型接触所采用的电子传输层（ETL）的改变来制造有效的平面N-I-P PSC。具体地，在钙钛矿沉积之前的氟基等离子体处理导致TiO的表面氟化 <sub> 2 </ sub> Etl。在TiO上存在氟 <sub> 2 </ sub> 表面大大改善了ALD层和甲基铅碘化碘钙钛矿膜之间的粘附性，并导致更有利的能带对准，伴随着界面处的更快的电子载体萃取。随着表面氟化的结果，我们观察到基于ALD的参考样品的电流密度 - 电压曲线滞后的显着降低，以及从4％的功率转换效率的显着提高到稳定的14.8％。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces 》</a> <b style="margin: 0 2px;">|</b><span>2018年第9期</span><b style="margin: 0 2px;">|</b> <span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zardetto Valerio&option=202" target="_blank" rel="nofollow">Zardetto Valerio;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=di Giacomo Francesco&option=202" target="_blank" rel="nofollow">di Giacomo Francesco;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lifka Herbert&option=202" target="_blank" rel="nofollow">Lifka Herbert;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Verheijen Marcel A.&option=202" target="_blank" rel="nofollow">Verheijen Marcel A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Weijtens Christ H. L.&option=202" target="_blank" rel="nofollow">Weijtens Christ H. L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Black Lachlan E.&option=202" target="_blank" rel="nofollow">Black Lachlan E.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Veenstra Sjoerd&option=202" target="_blank" rel="nofollow">Veenstra Sjoerd;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kessels Wilhelmus M. M.&option=202" target="_blank" rel="nofollow">Kessels Wilhelmus M. M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Andriessen Ronn&option=202" target="_blank" rel="nofollow">Andriessen Ronn;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Creatore Mariadriana&option=202" target="_blank" rel="nofollow">Creatore Mariadriana;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>TNO/Host/SollianceHigh Tech Campus 21 5656 AE Eindhoven The Netherlands;</p> <p>TNO/Host/SollianceHigh Tech Campus 21 5656 AE Eindhoven The Netherlands;</p> <p>TNO/Host/SollianceHigh Tech Campus 21 5656 AE Eindhoven The Netherlands;</p> <p>Philips Innovation LabsHigh Tech Campus 11 5656 AE Eindhoven The Netherlands;</p> <p>Department of Applied PhysicsEindhoven University of TechnologyP.O. Box 513 5600 MB Eindhoven The Netherlands;</p> <p>Department of Applied PhysicsEindhoven University of TechnologyP.O. Box 513 5600 MB Eindhoven The Netherlands;</p> <p>ECN/SollianceHigh Tech Campus 21 5656 AE Eindhoven The Netherlands;</p> <p>Department of Applied PhysicsEindhoven University of TechnologyP.O. Box 513 5600 MB Eindhoven The Netherlands;</p> <p>TNO/Host/SollianceHigh Tech Campus 21 5656 AE Eindhoven The Netherlands;</p> <p>Department of Applied PhysicsEindhoven University of TechnologyP.O. Box 513 5600 MB Eindhoven The Netherlands;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=CF 4 plasma&option=203" rel="nofollow">CF 4 plasma;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=low‐temperature atomic layer deposition&option=203" rel="nofollow">low‐temperature atomic layer deposition;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=perovskite&option=203" rel="nofollow">perovskite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=surface treatment&option=203" rel="nofollow">surface treatment;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=TiO 2&option=203" rel="nofollow">TiO 2;</a> </p> <div class="translation"> 机译：CF 4等离子体;低温原子层沉积;钙钛矿;表面处理;TiO 2; 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tuijian_authcolor">,孙伟海</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李昭&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,李昭</a> <span> <a href="/journal-cn-10701/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 发光学报 </a> </span> <span> . 2021</span><span> ,第005期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_materials-reports_thesis/0201211364021.html">用于钙钛矿太阳能电池光阳极的TiO2/ZnTiO3复合物的制备与性能</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=徐艳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 徐艳</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张翁晶&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张翁晶</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡木林&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,胡木林</a> <span> <a href="/journal-cn-7645/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 材料导报 </a> </span> <span> . 2016</span><span> ,第020期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-39109_thesis/020222432504.html">平面型高效率钙钛矿太阳能电池的研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=朱瑞&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 朱瑞</a> <span> <a href="/conference-cn-39109/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第十三届全国太阳级硅及光伏发电研讨会 </a> <span> <span> . 2017</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020312017203.html">基于TiO2@SnO2双电子传输层高效稳定钙钛矿太阳能电池的组分工程</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=顾浩&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 顾浩</a> <span> . 2018</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120113055011.html">一种钙钛矿太阳能电池TiO<Sub>2</Sub>电子传输层的制备方法</a> <b>[P]</b> . <span> 中国专利： CN113087012A </span> <span> . 2021-07-09</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061204005637.html">一种无电子传输层的平面钙钛矿太阳能电池的制备方法</a> <b>[P]</b> . <span> 中国专利： CN109119537B </span> <span> . 2020.09.18</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130408561701.html">Electron transporting layer for flexible perovskite solar cells and flexible perovskite solar cells including the same</a> <b>[P]</b> . <span> 外国专利：  KR101773972B1 </span> <span> . 2017-09-04</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于柔性钙钛矿太阳能电池的电子传输层以及包括该电子传输层的柔性钙钛矿太阳能电池 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130408795796.html">CYTOP Planar . Efficient life time planar Perovskite solar cells with CYTOP passivation layer and the method for fabricating thereof</a> <b>[P]</b> . <span> 外国专利：  KR20160139604A </span> <span> . 2016-12-07</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：CYTOP平面。具有CYTOP钝化层的高效寿命平面钙钛矿太阳能电池及其制造方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130402031752.html">Efficient and stable perovskite solar cells with all solution processed metal oxide transporting layers</a> <b>[P]</b> . <span> 外国专利：  US10693071B2 </span> <span> . 2020-06-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：高效稳定的钙钛矿型太阳能电池，具有所有溶液处理的金属氧化物传输层 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" 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Surface Fluorination of ALD TiO 22 Electron Transport Layer?for Efficient Planar Perovskite Solar Cells

摘要

Surface Fluorination of ALD TiO ₂2 Electron Transport Layer?for Efficient Planar Perovskite Solar Cells