Graphene Oxide/Carbon Nanotube Bilayer Flexible Membrane for High‐Performance Li–S Batteries with Superior Physical and Electrochemical Properties

Lee Dong Kyu; Kim Seon Joon; Kim Yong‐Jae; Choi Hyunji; Kim Dae Woo; Jeon Hwan‐Jin; Ahn Chi Won; Lee Jae W.; Jung Hee‐Tae

摘要

Abstract > Developing a highly effective interlayer inserted between the sulfur electrode and separator is one of the most important issues in Li–S battery research, because this interlayer enhances the cycle performance of the Li–S battery by trapping the lithium polysulfides in the sulfur electrode. Among various interlayer materials, carbon materials such as graphene and carbon nanotubes are particularly appealing because of their high electrical conductivity. Here, a new flexible carbon membrane interlayer consisting of graphene oxide (GO) and carbon nanotubes (CNTs) is developed by a facile vacuum filtration approach to trap the lithium polysulfides in the sulfur electrode. When the GO/CNT bilayer membrane is used as an interlayer between the sulfur electrode and separator (glass fiber), the Li–S battery delivers an initial discharge capacity of 1591.56 mAh g ?1 and maintains a capacity of about 1000?mAh?g ?1 over 50 cycles at 0.2C with a low potential difference of 150?mV. This reflects higher electrochemical performance than a GO or CNT monolayer unilaterally. This is attributed to the hydrophilic functional group of the GO layer strongly adsorbing lithium polysulfides dissolved in liquid electrolyte and the CNT layer enhancing the ion conductivity. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在硫电极和分离器之间形成高效的中间层是Li-S电池研究中最重要的问题之一，因为该中间层通过捕获硫电极中的锂多硫化物来增强Li-S电池的循环性能。在各种层间材料中，由于其高导电性，诸如石墨烯和碳纳米管的碳材料特别吸引。这里，由石墨烯（GO）和碳纳米管（CNT）组成的新的柔性碳膜夹层通过容易真空过滤方法开发，以捕获硫电极中的多硫化物。当GO / CNT双层膜用作硫电极和隔膜（玻璃纤维）之间的中间层时，LI-S电池可提供1591.56mAhg的初始放电容量？1 </ sup> 并保持容量约1000？Mah？G ？1 </ sup> 在0.2℃下超过50个循环，低电位差为150ΩmV。这反映了更高的电化学性能而不是单方面的Go或CNT单层。这归因于溶解在液体电解质中溶解在液体电解质中的脱脂锂多硫化物的亲水性官能团和增强离子电导率的CNT层。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2019年第7期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Dong Kyu&option=202" target="_blank" rel="nofollow">Lee Dong Kyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Seon Joon&option=202" target="_blank" rel="nofollow">Kim Seon Joon;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Yong‐Jae&option=202" target="_blank" rel="nofollow">Kim Yong‐Jae;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Choi Hyunji&option=202" target="_blank" rel="nofollow">Choi Hyunji;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Dae Woo&option=202" target="_blank" rel="nofollow">Kim Dae Woo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jeon Hwan‐Jin&option=202" target="_blank" rel="nofollow">Jeon Hwan‐Jin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ahn Chi Won&option=202" target="_blank" rel="nofollow">Ahn Chi Won;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Jae W.&option=202" target="_blank" rel="nofollow">Lee Jae W.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jung Hee‐Tae&option=202" target="_blank" rel="nofollow">Jung Hee‐Tae;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Wearable Platform Materials Technology CenterKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical Engineering and BiotechnologyKorea Polytechnic University237 Siheung‐si Gyeonggi‐do 15073 Republic of Korea;</p> <p>Department of Global Nanotechnology Development TeamNational Nanofab Center at Korea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> <p>Department of Chemical and Biomolecular EngineeringKorea Advanced Institute of Science and Technology (KAIST)Daejeon 34141 Republic of Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon nanotube&option=203" rel="nofollow">carbon nanotube;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=flexible membrane&option=203" rel="nofollow">flexible membrane;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=graphene oxide&option=203" rel="nofollow">graphene oxide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=interlayer&option=203" rel="nofollow">interlayer;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium–sulfur battery&option=203" rel="nofollow">lithium–sulfur battery;</a> </p> <div class="translation"> 机译：碳纳米管;柔性膜;石墨烯;层间;锂 - 硫磺电池; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022433829.html">Graphene Oxide/Carbon Nanotube Bilayer Flexible Membrane for High‐Performance Li–S 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href="/patent-detail/06120112478518.html">一种双层结构的聚3,4-乙烯二氧噻吩/氧化石墨烯-碳纳米管柔性透明导电薄膜及其制备方法</a> <b>[P]</b> . <span> 中国专利： CN112509729A </span> <span> . 2021-03-16</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120109083126.html">化学上稳定的烷基铝溶液、烷基铝水解组合物溶液、铝氧化物膜涂布形成用组合物、具有铝氧化物膜的物品、其制造方法、氧化铝薄膜的制造方法、钝化膜的制造方法、钝化膜、使用其的太阳能电池元件</a> <b>[P]</b> . <span> 中国专利： CN106573790A </span> <span> . 2017-04-19</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130406365602.html">GRAPHENE OXIDE/CARBON NANOTUBE COMPOSITE FIBER HAVING HETEROJUNCTION STRUCTURE, AND METHOD FOR MANUFACTURING GRAPHENE OXIDE/GRAPHENE COMPOSITE FIBER OR GRAPHENE OXIDE/GRAPHENE/CARBON NANOTUBE COMPOSITE FIBER</a> <b>[P]</b> . <span> 外国专利：  WO2018004099A1 </span> <span> . 2018-01-04</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> 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