Interface and Morphology Control of the Thermal Conductivity in Core–Shell Particle Colloidal Crystals

Ruckdeschel Pia; Retsch Markus

摘要

Abstract >The thermal transport properties of nanostructured composite colloidal assemblies are investigated. These are of importance for future phase change material applications, which increasingly address the micrometer and sub‐micrometer ranges. Polystyrene silica core–shell colloidal particles sizes of 270–480 nm and shell thicknesses of 15–42 nm are used as a structurally well?defined model system. This allows deducing precise structure property relationships with the lowest thermal conductivity being observed for particles with a large diameter, a thin shell thickness, and the highest polymer content. Importantly, clear evidence is found for polymer leakage through 15 nm silica shells when exceeding the glass transition temperature of the core polymer. This leads to a steady increase in thermal conductivity but also presents a lower limit for the silica shell thickness to contain the second phase. For a complete understanding, the findings are discussed in the light of colloidal crystals consisting of pure silica and polystyrene particles. Solid silica sphere colloidal crystals possess the highest thermal conductivity, and pure polymer beads the lowest. This demonstrates to which extent the thermal transport properties can be solely adjusted by the particle composition and morphology. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >研究了纳米结构复合胶体组件的热传输性能。这些对未来相变材料应用的重要性是重要的，这越来越多地解决了千分尺和亚微米的范围。聚苯乙烯二氧化硅芯 - 壳胶体颗粒尺寸为270-480nm，壳体厚度为15-42nm，用作结构良好的模型系统。这允许用大直径，薄壳厚度和最高聚合物含量的颗粒观察到精确的结构性质关系。重要的是，当超过核心聚合物的玻璃化转变温度时，发现通过15nm二氧化硅壳的聚合物泄漏发现清晰的证据。这导致导热率稳定增加，但也呈现了二氧化硅壳厚度的下限以含有第二相。为了完全理解，根据由纯二氧化硅和聚苯乙烯颗粒组成的胶体晶体来讨论发现。固体二氧化硅球胶体晶体具有最高的导热性，纯聚合物珠粒最低。这证明了热传输性能可以单独调节颗粒组成和形态学的程度。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2017年第24期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ruckdeschel Pia&option=202" target="_blank" rel="nofollow">Ruckdeschel Pia;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Retsch Markus&option=202" target="_blank" rel="nofollow">Retsch Markus;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Physical Chemistry Polymer SystemsUniversity of BayreuthUniversitaetsstr. 30 95447 Bayreuth Germany;</p> <p>Physical Chemistry Polymer SystemsUniversity of BayreuthUniversitaetsstr. 30 95447 Bayreuth Germany;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hierarchical mesostructure&option=203" rel="nofollow">hierarchical mesostructure;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoporous material&option=203" rel="nofollow">nanoporous material;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=phase change material&option=203" rel="nofollow">phase change material;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thermal contact resistance&option=203" rel="nofollow">thermal contact resistance;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=thermal diffusivity&option=203" rel="nofollow">thermal diffusivity;</a> </p> <div class="translation"> 机译：分层介质;纳米孔材料;相变材料;热接触电阻;热扩散率; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022433782.html">Interface and Morphology Control of the Thermal Conductivity in Core–Shell Particle Colloidal Crystals</a> <b>[J]</b> . <span> <a 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