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首页> 外文期刊>Advanced materials interfaces >Entropy‐Maximized Synthesis of Multimetallic Nanoparticle Catalysts via a Ultrasonication‐Assisted Wet Chemistry Method under Ambient Conditions
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Entropy‐Maximized Synthesis of Multimetallic Nanoparticle Catalysts via a Ultrasonication‐Assisted Wet Chemistry Method under Ambient Conditions

机译：在环境条件下通过超声辅助湿化学方法熵最大化的多金属纳米颗粒催化剂的合成

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Abstract > A facile ultrasonication‐assisted wet chemistry method for preparing multicomponent alloy nanoparticles (NPs) including high‐entropy alloys (HEAs) is reported. PtAuPdRhRu alloy (HEA), quaternary PtAuPdRh alloy, and ternary PtAuPd alloy NPs are produced with ≈3 nm in diameter. Taking advantage of the acoustic cavitation phenomenon in ultrasonication process, noble metal precursors could be co‐reduced by chemical reductants and transform to alloy structures under operation at room conditions. The instantaneous massive energy (≈5000 °C, 2000 atm) occurring in momentary timespans (≤10 ?9 s) contributes to the formation of multimetallic mixed nanomaterials driven by entropy maximization. Owing to strong synergistic effects, the catalysts with the HEA NPs supported on carbons exhibit prominent electrocatalytic activities for hydrogen evolution reaction. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 报道了一种用于制备包括高熵合金（HEAS）的多组分合金纳米颗粒（NPS）的容易的超声辅助湿化学方法。 PTAUPDRHRU合金（HEA），季型PTAUPDRH合金和三元PTAUPD合金NPS在直径≈3纳米的直径下产生。利用超声过程中的声学空化现象，通过化学还原剂可以共同减少贵金属前体，并在室内条件下在操作下转化为合金结构。在瞬时的时间表（≤10）中发生瞬时大量能量（≈5000°C，2000 ATM）（≤10 ？9 </ sup> S）有助于形成由熵最大化驱动的多金属混合纳米材料。由于强烈的协同作用，碳碳的催化剂具有碳的HEA NPS表现出突出的电催化活性为氢化反应。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2019年第7期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Miaomiao&option=202" target="_blank" rel="nofollow">Liu Miaomiao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Zihao&option=202" target="_blank" rel="nofollow">Zhang Zihao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Okejiri Francis&option=202" target="_blank" rel="nofollow">Okejiri Francis;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Shize&option=202" target="_blank" rel="nofollow">Yang Shize;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhou Shenghu&option=202" target="_blank" rel="nofollow">Zhou Shenghu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dai Sheng&option=202" target="_blank" rel="nofollow">Dai Sheng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237 China;</p> <p>Department of ChemistryThe University of Tennessee KnoxvilleKnoxville TN 37996 USA;</p> <p>Department of ChemistryThe University of Tennessee KnoxvilleKnoxville TN 37996 USA;</p> <p>Center for Functional NanomaterialsBrookhaven National LaboratoryUpton NY 11973 USA;</p> <p>School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237 China;</p> <p>Department of ChemistryThe University of Tennessee KnoxvilleKnoxville TN 37996 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=alkaline HER&option=203" rel="nofollow">alkaline HER;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=high‐entropy alloy&option=203" rel="nofollow">high‐entropy alloy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoparticles&option=203" rel="nofollow">nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ultrasonication‐assisted&option=203" rel="nofollow">ultrasonication‐assisted;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=wet chemistry method&option=203" rel="nofollow">wet chemistry method;</a> </p> <div class="translation"> 机译：碱性她;高熵合金;纳米粒子;超声波辅助;湿化学方法; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022433732.html">Entropy‐Maximized Synthesis of Multimetallic Nanoparticle Catalysts via a 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