Intense Vibronic Modulation of the Chiral Photoelectron Angular Distribution Generated by Photoionization of Limonene Enantiomers with Circularly Polarized Synchrotron Radiation

Rafiee?Fanood Mohammad M.; Ganjitabar Hassan; Garcia Gustavo A.; Nahon Laurent; Turchini Stefano; Powis Ivan

摘要

Abstract >Photoionization of the chiral monoterpene limonene has been investigated using polarized synchrotron radiation between the adiabatic ionization threshold, 8.505 and 23.5?eV. A rich vibrational structure is seen in the threshold photoelectron spectrum and is interpreted using a variety of computational methods. The corresponding photoelectron circular dichroism—measured in the photoelectron angular distribution as a forward–backward asymmetry with respect to the photon direction—was found to be strongly dependent on the vibronic structure appearing in the photoelectron spectra, with the observed asymmetry even switching direction in between the major vibrational peaks. This effect can be ultimately attributed to the sensitivity of this dichroism to small phase shifts between adjacent partial waves of the outgoing photoelectron. These observations have implications for potential applications of this chiroptical technique, where the enantioselective analysis of monoterpene components is of particular interest. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>摘要</标题> >在绝热电离阈值之间使用偏振同步辐射进行了手性单萜烯酮的光偶联， 8.505和23.5？EV。在阈值光电子谱中看到富振动结构，并使用各种计算方法解释。在光电子角分布中测量的相应光电子圆形二色二分 - 发现相对于光子方向的前后不对称 - 被发现强烈地取决于出现在光电子谱中的振动结构，观察到的不对称性甚至切换方向主要的振动峰。这种效果最终可能归因于该二分波动对传出光电子的相邻部分波之间的小相移的敏感性。这些观察结果对该阴压技术的潜在应用有影响，其中单萜组分的对映选择性分析特别感兴趣。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16300/'>《Chemphyschem: A European journal of chemical physics and physical chemistry》</a> <b style="margin: 0 2px;">|</b><span>2018年第8期</span><b style="margin: 0 2px;">|</b><span>共13页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Rafiee?Fanood Mohammad M.&option=202" target="_blank" rel="nofollow">Rafiee?Fanood Mohammad M.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ganjitabar Hassan&option=202" target="_blank" rel="nofollow">Ganjitabar Hassan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Garcia Gustavo A.&option=202" target="_blank" rel="nofollow">Garcia Gustavo A.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nahon Laurent&option=202" target="_blank" rel="nofollow">Nahon Laurent;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Turchini Stefano&option=202" target="_blank" rel="nofollow">Turchini Stefano;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Powis Ivan&option=202" target="_blank" rel="nofollow">Powis Ivan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>LaserLaB AmsterdamVU University AmsterdamDe Boelelaan 1081 1081 HV Amsterdam The Netherlands;</p> <p>School of ChemistryThe University of NottinghamUniversity Park Nottingham NG7 2RD UK;</p> <p>Synchrotron SOLEILl'Orme des Merisiers Saint Aubin BP 48 91192 Gif sur Yvette Cedex France;</p> <p>Synchrotron SOLEILl'Orme des Merisiers Saint Aubin BP 48 91192 Gif sur Yvette Cedex France;</p> <p>Istituto Struttura della Materia-CNR (ISM-CNR)Via del Fosso del Cavaliere 100 00133 Roma Italy;</p> <p>School of ChemistryThe University of NottinghamUniversity Park Nottingham NG7 2RD UK;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=chirality&option=203" rel="nofollow">chirality;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=molecular photoionization dynamics&option=203" rel="nofollow">molecular photoionization dynamics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photoelectron&option=203" rel="nofollow">photoelectron;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=synchrotron radiation&option=203" rel="nofollow">synchrotron radiation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=terpenes&option=203" rel="nofollow">terpenes;</a> </p> <div class="translation"> 机译：手性;分子光离子动态;光电子;同步辐射;Terpenes; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a 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2007</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/02031633343.html">分子和自由基的同步辐射光电子光离子符合实验研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=朱宇鹏&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 朱宇鹏</a> <span> . 2017</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061204467952.html">具有可调节的非圆形驱动元件的同步传动装置</a> <b>[P]</b> . <span> 中国专利： CN110088433B </span> <span> . 2021.06.15</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120101105725.html">具有可调节的非圆形驱动元件的同步传动装置</a> <b>[P]</b> . <span> 中国专利： CN110088433A </span> <span> . 2019-08-02</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130480760031.html">A device for converting circularly polarized radiation in linearly polarized radiation having a rotating plane of polarization at a constant angular speed</a> <b>[P]</b> . <span> 外国专利：  DE000001797378C3 </span> <span> . 1977-11-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：一种用于将圆偏振辐射转换为具有恒定角速度的偏振旋转平面的线偏振辐射的装置 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130481792891.html">A device for converting circularly polarized radiation in linearly polarized radiation having a rotating plane of polarization at a constant angular speed</a> <b>[P]</b> . <span> 外国专利：  DE1797378B2 </span> <span> . 1977-03-24</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：一种用于将圆偏振辐射转换为具有恒定角速度的偏振旋转平面的线偏振辐射的装置 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130487347000.html">A device for converting circularly polarized radiation in linearly polarized radiation having a rotating plane of polarization at a constant angular speed</a> <b>[P]</b> . <span> 外国专利：  DE1797378A1 </span> <span> . 1971-08-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：一种用于将圆偏振辐射转换为具有恒定角速度的偏振旋转平面的线偏振辐射的装置 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022115217','4',7,2,1,'',this,24)" class="delivery" 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