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首页> 外文期刊>Chemistry, an Asian journal >Triphenylamine–Thienothiophene Organic Charge‐Transport Molecular Materials: Effect of Substitution Pattern on their Thermal, Photoelectrochemical, and Photovoltaic Properties
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Triphenylamine–Thienothiophene Organic Charge‐Transport Molecular Materials: Effect of Substitution Pattern on their Thermal, Photoelectrochemical, and Photovoltaic Properties

机译：三苯胺 - Thienthishiophene有机电荷运输分子材料：替代图案对其热，光电化学和光伏性能的影响

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Abstract > Two readily accessible thienothiophene–triphenylamine charge‐transport materials have been synthesized by simply varying the substitution pattern of the triphenylamine groups on a central thienothiophene π‐linker. The impact of the substitution pattern on the thermal, photoelectrochemical, and photovoltaic properties of these materials was evaluated and, based on theoretical and experimental studies, we found that the isomer in which the triphenylamine groups were located at the 2,5‐positions of the thienothiophene core ( TT‐2,5‐TPA ) had better π‐conjugation than the 3,6‐isomer ( TT‐3,6‐TPA ). Whilst the thermal, morphological, and hydrophobic properties of the two materials were similar, their optoelectrochemical and photovoltaic properties were noticeably impacted. When applied as hole‐transport materials in hybrid perovskite solar cells, the 2,5‐isomer exhibited a power‐conversion efficiency of 13.6?%, much higher than that of its 3,6‐counterpart (0.7?%) under the same standard conditions. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> > 通过简单地改变在中央Thienhiopheneπ-Linker上的三苯胺基团的替代模式，已经合成了两种容易访问的噻吩丙胺 - 三苯胺电荷转运材料。评估替代模式对这些材料的热，光电化学和光伏性能的影响，并基于理论和实验研究，我们发现三苯胺基团位于2,5位的异构体Thienothiophene核心（ <B> TT-2,5-TPA </ B> ）具有比3,6-异构体更好的π-缀合（ tt-3,6-tpa </ b> ）。虽然两种材料的热，形态和疏水性质相似，但它们的光电子化学和光伏性能明显受到影响。当在杂交钙钛矿太阳能电池中施加作为空穴传输材料时，2,5异构体表现出13.6μm的功率转换效率，远高于相同标准下的3,6-对应物（0.7℃）的功率转换效率状况。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16161/'>《Chemistry, an Asian journal》</a> <b style="margin: 0 2px;">|</b><span>2018年第10期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Le Thi Huong&option=202" target="_blank" rel="nofollow">Le Thi Huong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dao Quang‐Duy&option=202" target="_blank" rel="nofollow">Dao Quang‐Duy;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Nghiêm Mai‐Phuong&option=202" target="_blank" rel="nofollow">Nghiêm Mai‐Phuong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Péralta Sébastien&option=202" target="_blank" rel="nofollow">Péralta Sébastien;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guillot Regis&option=202" target="_blank" rel="nofollow">Guillot Regis;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pham Quoc Nghi&option=202" target="_blank" rel="nofollow">Pham Quoc Nghi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fujii Akihiko&option=202" target="_blank" rel="nofollow">Fujii Akihiko;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ozaki Masanori&option=202" target="_blank" rel="nofollow">Ozaki Masanori;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Goubard Fabrice&option=202" target="_blank" rel="nofollow">Goubard Fabrice;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bui Thanh‐Tuan&option=202" target="_blank" rel="nofollow">Bui Thanh‐Tuan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Laboratoire de Physicochimie des Polymères et des InterfacesUniversité de Cergy-Pontoise5 mail Gay Lussac 95000 Neuville-sur-Oise France;</p> <p>Division of Electrical Electronic and Informational EngineeringOsaka University2-1 Yamada-oka Suita-shi Osaka-fu 565-0871 Japan;</p> <p>Plateforme Microscopies et AnalysesUniversité de Cergy-PontoiseRue Descartes 95000 Neuville-sur-Oise France;</p> <p>Laboratoire de Physicochimie des Polymères et des InterfacesUniversité de Cergy-Pontoise5 mail Gay Lussac 95000 Neuville-sur-Oise France;</p> <p>Institut de Chimie Moléculaire et des Matériaux d'Orsay CNRSUniversité Paris Sud91405 Orsay Cedex France;</p> <p>Institut de Chimie Moléculaire et des Matériaux d'Orsay CNRSUniversité Paris Sud91405 Orsay Cedex France;</p> <p>Division of Electrical Electronic and Informational EngineeringOsaka University2-1 Yamada-oka Suita-shi Osaka-fu 565-0871 Japan;</p> <p>Division of Electrical Electronic and Informational EngineeringOsaka University2-1 Yamada-oka Suita-shi Osaka-fu 565-0871 Japan;</p> <p>Laboratoire de Physicochimie des Polymères et des InterfacesUniversité de Cergy-Pontoise5 mail Gay Lussac 95000 Neuville-sur-Oise France;</p> <p>Laboratoire de Physicochimie des Polymères et des InterfacesUniversité de Cergy-Pontoise5 mail Gay Lussac 95000 Neuville-sur-Oise France;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hole-transport materials&option=203" rel="nofollow">hole-transport materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=materials science&option=203" rel="nofollow">materials science;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nitrogen heterocycles&option=203" rel="nofollow">nitrogen heterocycles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=solar cells&option=203" rel="nofollow">solar cells;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sulfur heterocycles&option=203" rel="nofollow">sulfur heterocycles;</a> </p> <div class="translation"> 机译：空穴传输材料;材料科学;氮杂环;太阳能电池;硫杂环; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022087192.html">Triphenylamine–Thienothiophene Organic Charge‐Transport Molecular Materials: Effect of Substitution Pattern on their Thermal, Photoelectrochemical, and Photovoltaic Properties</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Le Thi Huong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Le Thi Huong,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dao Quang‐Duy&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dao Quang‐Duy,</a> <a 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