Cuboid Ni <sub xmlns='http://www.wiley.com/namespaces/wiley'>2</sub>2 P as a Bifunctional Catalyst for Efficient Hydrogen Generation from Hydrolysis of Ammonia Borane and Electrocatalytic Hydrogen Evolution

Du Yeshuang; Liu Chao; Cheng Gongzhen; Luo Wei

摘要

Abstract > The design of high‐performance catalysts for hydrogen generation is highly desirable for the upcoming hydrogen economy. Herein, we report the colloidal synthesis of nanocuboid Ni <sub>2</sub> P by the thermal decomposition of nickel chloride hexahydrate (NiCl <sub>2</sub> ? 6?H <sub>2</sub> O) and trioctylphosphine. The obtained nanocuboid Ni <sub>2</sub> P was characterized by using powder X‐ray diffraction, transmission electron microscopy, energy‐dispersive X‐ray spectroscopy, X‐ray photoelectron spectroscopy, and inductively coupled plasma atomic emission spectroscopy. For the first time, the as‐synthesized nanocuboid Ni <sub>2</sub> P is used as a bifunctional catalyst for hydrogen generation from the hydrolysis of ammonia borane and electrocatalytic hydrogen evolution. Owing to the strong synergistic electronic effect between Ni and P, the as‐synthesized Ni <sub>2</sub> P exhibits catalytic performance that is superior to its counterpart without P doping. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >设计对于即将到来的氢气经济性，高效催化剂的高效催化剂非常适合。在此，我们通过镍氯化镍六水合物的热分解报告纳米吡吡吡喃镓Ni <sub> 2 /亚> p的胶体合成（NiCl <sub> 2 </ sub> 6Ω·h <sub > 2 </ sub> O）和三辛基膦。通过使用粉末X射线衍射，透射电子显微镜，能量分散X射线光谱，X射线光电子体光谱和电感耦合等离子体原子发射光谱，所以所得纳米吡吡吡吡吡替纳氏乳蛋白酶2/ 2 </ sub> P。首次首次，用作氨硼烷水解和电催化氢进化的氢气的双官能催化剂用作双官能催化剂。由于Ni和P之间的强度协同电子效果，AS合成的Ni <sub> 2 </ sub> P表现出优于其对应物而没有P掺杂的催化性能。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16161/'>《Chemistry, an Asian journal 》</a> <b style="margin: 0 2px;">|</b><span>2017年第22期</span><b style="margin: 0 2px;">|</b> <span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Yeshuang&option=202" target="_blank" rel="nofollow">Du Yeshuang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Chao&option=202" target="_blank" rel="nofollow">Liu Chao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cheng Gongzhen&option=202" target="_blank" rel="nofollow">Cheng Gongzhen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Luo Wei&option=202" target="_blank" rel="nofollow">Luo Wei;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>College of Chemistry and Molecular SciencesWuhan UniversityWuhan Hubei 430072 P. R. China;</p> <p>College of Chemistry and Molecular SciencesWuhan UniversityWuhan Hubei 430072 P. R. China;</p> <p>College of Chemistry and Molecular SciencesWuhan UniversityWuhan Hubei 430072 P. R. China;</p> <p>College of Chemistry and Molecular SciencesWuhan UniversityWuhan Hubei 430072 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=boranes&option=203" rel="nofollow">boranes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrochemistry&option=203" rel="nofollow">electrochemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogen&option=203" rel="nofollow">hydrogen;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanostructures&option=203" rel="nofollow">nanostructures;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=transition-metal phosphides&option=203" rel="nofollow">transition-metal phosphides;</a> </p> <div class="translation"> 机译：硼烷;电化学;氢;纳米结构;过渡金属磷化物; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022087022.html">Cuboid Ni <sub xmlns="http://www.wiley.com/namespaces/wiley">2</sub>2 P as a Bifunctional Catalyst for Efficient 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Cuboid Ni 22 P as a Bifunctional Catalyst for Efficient Hydrogen Generation from Hydrolysis of Ammonia Borane and Electrocatalytic Hydrogen Evolution

摘要

Cuboid Ni ₂2 P as a Bifunctional Catalyst for Efficient Hydrogen Generation from Hydrolysis of Ammonia Borane and Electrocatalytic Hydrogen Evolution