An Investigation into the Charge‐Storage Mechanism of MnO@Graphite as Anode for Lithium‐Ion Batteries at Low Temperature

Tian Xiaodong; Du Li; Yan Yurong; Wu Songping

摘要

Abstract > Electrochemical features and the charge‐storage mechanism of monodispersed MnO nanoparticles anchored on graphite (MnO@Graphite) for Li‐ion batteries have been investigated at a low‐temperature of ?25?°C. MnO@Graphite nanocomposite rendered a remarkable reversible capacity of 456?mA h g ?1 after 320 cycles under a current density of 100?mA?g ?1 at such a low temperature. Remarkable reversible capacity could be ascribed to the integrated structure, emergence of in‐situ formed MnO <sub>2</sub> and hybrid pseudocapacitance. Hybrid pseudocapacitive contributions have appeared at low operational temperature, i.?e., assembled heterogeneous intercalation pseudocapacitance at low potentials and surface‐controlled pseudocapacitance at high potentials. The results showed that the prepared MnO@Graphite nanocomposite is a promising candidate for Li‐ion batteries operated in harsh environment. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在低温的α25℃下研究了锚定石墨（MNO @石墨）的单分散MNO纳米粒子的电化学特征和电荷储存机理。 MNO @石墨纳米复合材料呈现出显着的可逆容量为456？MA H G. ？1 </ sup> 在电流密度为100Ωma的320次循环之后？1 </ sup> 在这种低温下。可逆的可逆能力可以归因于综合结构，出现原位形成的MNO <sub> 2 </ sub> 和杂交伪宽度。 Hybrid Pseudocapactive贡献已经出现在低运行温度下，I.?E。，在低电位下，在低电位和表面控制的假偶联处组装的异质插入假偶像。结果表明，制备的MNO @石墨纳米复合材料是在恶劣环境中操作的锂离子电池的有望候选者。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第8期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Xiaodong&option=202" target="_blank" rel="nofollow">Tian Xiaodong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Li&option=202" target="_blank" rel="nofollow">Du Li;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Yurong&option=202" target="_blank" rel="nofollow">Yan Yurong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Songping&option=202" target="_blank" rel="nofollow">Wu Songping;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510641 China;</p> <p>School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510641 China;</p> <p>School of Materials Science and EngineeringSouth China University of TechnologyGuangzhou 510641 China;</p> <p>School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510641 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=anode material&option=203" rel="nofollow">anode material;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=composite materials&option=203" rel="nofollow">composite materials;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=low temperature&option=203" rel="nofollow">low temperature;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-ion batteries&option=203" rel="nofollow">lithium-ion batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=pseudocapacitance&option=203" rel="nofollow">pseudocapacitance;</a> </p> <div class="translation"> 机译：阳极材料;复合材料;低温;锂离子电池;假偶像; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022060820.html">An Investigation into the Charge‐Storage Mechanism of MnO@Graphite as Anode for Lithium‐Ion Batteries at Low Temperature</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Xiaodong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Tian Xiaodong,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Du Li&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Du Li,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Yurong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yan Yurong,</a> <a href="/journal-foreign-16042/" target="_blank" rel="nofollow" class="tuijian_authcolor">ChemElectroChem .</a> <span>2019</span><span>,第8期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：MNO @石墨电荷储存机制作为低温下锂离子电池阳极的电荷储存机理研究</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704018474133.html">High-performance Sn@carbon nanocomposite anode for lithium-ion batteries: Lithium storage processes characterization and low-temperature behavior</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=F. 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