Phosphorus and Boron Co‐Doped Carbon Coating of LiNi0.5Mn1.5O4 Cathodes for Advanced Lithium‐ion Batteries

Gu Tingting; Wang Jin; Tian Jing‐Hua; Zheng Xiangjun; Lu Kewei; Xin Yu; Wang Haibo; Yang Ruizhi

摘要

Abstract > A facile approach for the preparation of phosphorus and boron co‐doped carbon coated LiNi <sub>0.5</sub> Mn <sub>1.5</sub> O <sub>4</sub> , which is then applied as cathode materials for lithium ion batteries has been investigated. The effect of carbon coating amounts on the battery performance has been studied systematically. The 5?wt.% carbon coated sample exhibits the most outstanding performance, including an excellent capacity retention of 96.7?% after 200 cycles, superior rate capability (111?mAh?g ?1 capacity at 5?C), and significantly improved cycle life under 1?C. It is believed that the phosphorus and boron co‐doped carbon coating layer could suppress side‐reactions between the electrolyte and LiNi <sub>0.5</sub> Mn <sub>1.5</sub> O <sub>4</sub> , and alleviate the dissolution of manganese ions into the electrolyte effectively. Moreover, electrochemical impedance spectroscopy results reveal that the phosphorus and boron co‐doped carbon coating on LiNi <sub>0.5</sub> Mn <sub>1.5</sub> O <sub>4</sub> could reduce the charge transfer resistance significantly. The composite cathode therefore provides good conductivity as well as fast Li‐ion diffusion, then resulting in better rate capability and cycle life, even under a high temperature of 55?°C. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 一种磷和硼共掺杂碳涂层锂制备的容易方法 <sub> 0.5 </ sub> MN. <sub> 1.5 </ sub> O. <sub> 4 </ sub> 然后，已经研究了作为锂离子电池的阴极材料的应用。系统地研究了碳涂布量对电池性能的影响。 5？重量％。％碳涂层样品表现出最出色的性能，包括200个周期，优越的速率能力（111？MAH？MAH ？1 </ sup> 容量为5？c），并在1℃下显着改善循环寿命。据信，磷和硼共掺杂的碳涂层可以抑制电解质和亚麻之间的副反应 <sub> 0.5 </ sub> MN. <sub> 1.5 </ sub> O. <sub> 4 </ sub> ，并减轻有效地将锰离子溶解到电解质中。此外，电化学阻抗光谱结果表明，磷和硼共掺杂碳涂层 <sub> 0.5 </ sub> MN. <sub> 1.5 </ sub> O. <sub> 4 </ sub> 可以显着降低电荷转移阻力。因此，复合阴极提供良好的导电性以及快速锂离子扩散，然后导致更好的速率和循环寿命，即使在55Ω℃的高温下也会导致循环寿命。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第8期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gu Tingting&option=202" target="_blank" rel="nofollow">Gu Tingting;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Jin&option=202" target="_blank" rel="nofollow">Wang Jin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Jing‐Hua&option=202" target="_blank" rel="nofollow">Tian Jing‐Hua;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zheng Xiangjun&option=202" target="_blank" rel="nofollow">Zheng Xiangjun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lu Kewei&option=202" target="_blank" rel="nofollow">Lu Kewei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xin Yu&option=202" target="_blank" rel="nofollow">Xin Yu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Haibo&option=202" target="_blank" rel="nofollow">Wang Haibo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Ruizhi&option=202" target="_blank" rel="nofollow">Yang Ruizhi;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>School of Physical Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> <p>College of Energy Soochow Institute for Energy and Materials InnovationS &</p> <p>Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215006 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon coating&option=203" rel="nofollow">carbon coating;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=high voltage&option=203" rel="nofollow">high voltage;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=LiNi0.5Mn1.5O4&option=203" rel="nofollow">LiNi0.5Mn1.5O4;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium-ion batteries&option=203" rel="nofollow">lithium-ion batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=P&option=203" rel="nofollow">P;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=B co-doped&option=203" rel="nofollow">B co-doped;</a> </p> <div class="translation"> 机译：碳涂层;高压;LINI0.5MN1.5O4;锂离子电池;P;b共掺杂; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_transactions-nonferrous-metals-society-china_thesis/0201223133195.html">Na+掺杂对锂离子电池正极材料LiNi0.5Mn1.5O4晶体结构和电化学性能的影响</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王江峰&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">王江峰,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陈丹&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">陈丹,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=吴伟&option=202" target="_blank" rel="nofollow" class="tuijian_auth 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=聂平&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,聂平</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=薛向欣&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,薛向欣</a> <span> <a href="/journal-cn-4549/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 吉林师范大学学报（自然科学版） </a> </span> <span> . 2020</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_chemical-journal-chinese-universities_thesis/0201275816752.html">氮掺杂碳磷锂离子电池复合负极材料的制备及电化学性能</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李向南&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李向南</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=于明明&option=202" target="_blank" rel="nofollow" class="tuijian_auth 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<span> <span> . 2017</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020313562102.html">磷掺杂氮化硼/碳复合结构的制备及其在锂硫电池中的应用</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张璟&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张璟</a> <span> . 2019</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120113434982.html">一种碳磷硼三元共掺杂铜/镍基催化剂的制备方法及其应用</a> <b>[P]</b> . <span> 中国专利： CN113457728A </span> <span> . 2021-10-01</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120111661888.html">一种硼-氮-磷三元掺杂无金属碳材料及其制备方法和应用</a> <b>[P]</b> . <span> 中国专利： CN111613801A </span> <span> . 2020-09-01</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130500613454.html">PRISMATIC LITHIUM-ION BATTERY WITH A CATHODE BASED 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