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Atomically Dispersed Bimetallic FeNi Catalysts as Highly Efficient Bifunctional Catalysts for Reversible Oxygen Evolution and Oxygen Reduction Reactions

机译：原子上分散的双金属Feni催化剂作为高效的双官能催化剂，用于可逆氧气进化和氧还原反应

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Abstract > Bimetallic atomically dispersed FeNi catalysts anchored on N‐doped carbon nanotube with catalyst loading of 2–7?wt?% with different Fe?:?Ni ratio have been developed as highly active and stable bifunctional catalyst for reversible oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) for metal air batteries via a modified one‐pot synthesis method. Compared with atomically dispersed single Fe and Ni catalysts, the bimetallic FeNi catalysts exhibit outstanding performance for reversible OER and ORR, achieving a low potential gap (Δ E ) of 0.81?V to deliver an OER current density of 10?mA?cm ?2 and an ORR current density of 3?mA?cm ?2 . The FeNi electrodes also show a much better stability in the cyclic tests, compared to that of the state‐of‐the‐art Pt/C and Pt/C+Ir/C electrodes for reversible OER and ORR. The high performance is likely due to the significantly enhanced OER activity contributed by the introduction of Ni atoms, forming bridged FeNi bimetallic dual atom active sites for OER. This study provides a new platform for the development of highly active bimetallic atomic catalysts based bifunctional electrocatalysts for metal‐air batteries. The modified one‐pot synthesis methods demonstrated in this study can also be applicable to other atomically dispersed catalysts on CNTs or graphenes. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 双金属原子原子分散的Feni催化剂在N掺杂的碳纳米管上锚定，催化剂负载为2-7〜0·wtα％，不同的Fe？：Δni比为高活性和稳定的双官能催化剂，用于可逆氧还原反应（ORR）和通过改性单盆合成方法对金属空气电池的氧气进化反应（OER）。与原子分散的单氢和Ni催化剂相比，双金属FENI催化剂对可逆闭合孔和ORR具有出色的性能，实现了低潜在的间隙（δ e </ i> ）0.81？v以提供10？ma的oer电流密度？2 </ sup> 和orr电流密度为3？ma？cm ？2 </ sup> 。与用于可逆OER和ORR的最先进的PT / C和PT / C + IR / C电极相比，FENI电极在循环试验中也显示出更好的稳定性。高性能可能是由于通过引入Ni原子的贡献而产生的显着增强的OER活动，形成了OER的桥接FENI双原子活跃点。该研究为开发用于金属气电池的基于高活性双金属原子催化剂的高活性双金属原子催化剂的新平台。在该研究中证明的改性的单壶合成方法也可以应用于CNT或石墨烯上的其他原子分散的催化剂。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第13期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cheng Yi&option=202" target="_blank" rel="nofollow">Cheng Yi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Shuai&option=202" target="_blank" rel="nofollow">He Shuai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Veder Jean‐Pierre&option=202" target="_blank" rel="nofollow">Veder Jean‐Pierre;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=De?Marco Roland&option=202" target="_blank" rel="nofollow">De?Marco Roland;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Shi‐ze&option=202" target="_blank" rel="nofollow">Yang Shi‐ze;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ping?Jiang San&option=202" target="_blank" rel="nofollow">Ping?Jiang San;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Environmental EngineeringSchool of Metallurgy and Environment Central South UniversityChangsha 410083 China.;</p> <p>Fuels and Energy Technology Institute &</p> <p>Western Australia School of Mines: Minerals Energy and Chemical EngineeringCurtin University PerthWA 6102 Australia;</p> <p>John de Laeter CentreCurtin UniversityPerth WA 6102 Australia;</p> <p>Faculty of Science Health Education and EngineeringUniversity of Sunshine Coast Maroochydore DCQLD 4558 Australia;</p> <p>Materials Science and Technology DivisionOak Ridge National Laboratory Oak RidgeTN 37831 United States;</p> <p>Fuels and Energy Technology Institute &</p> <p>Western Australia School of Mines: Minerals Energy and Chemical EngineeringCurtin University PerthWA 6102 Australia;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=bifunctional catalysts&option=203" rel="nofollow">bifunctional catalysts;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen reduction reaction&option=203" rel="nofollow">oxygen reduction reaction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen evolution reaction&option=203" rel="nofollow">oxygen evolution reaction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=bimetallic catalysts&option=203" rel="nofollow">bimetallic catalysts;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal air batteries&option=203" rel="nofollow">metal air batteries;</a> </p> <div class="translation"> 机译：双官能催化剂;氧还原反应;氧气进化反应;双金属催化剂;金属空气电池; 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