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首页> 外文期刊>ChemCatChem >Zwitterionic Imidazole‐Urea Derivative Framework Bridged Mesoporous Hybrid Silica: A Highly Efficient Heterogeneous Nanocatalyst for Carbon Dioxide Conversion
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Zwitterionic Imidazole‐Urea Derivative Framework Bridged Mesoporous Hybrid Silica: A Highly Efficient Heterogeneous Nanocatalyst for Carbon Dioxide Conversion

机译：两性离子咪唑 - 尿素衍生物框架桥接介孔杂交二氧化硅：用于二氧化碳转化的高效非均相纳米催化剂

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Abstract > The use of supported zwitterionic nanoparticles is an interesting and important strategy for the development of new CO <sub>2</sub> conversion catalysts with enhanced activity and selectivity. Several zwitterionic imidazole‐urea derivative frameworks bridged mesoporous hybrid silica materials were prepared and characterized by using FTIR spectroscopy, solid‐state NMR spectroscopy, X‐ray photoelectron spectroscopy, XRD, TEM, and thermogravimetric analysis. The new Im‐Si‐X‐? materials possess a high surface area, hydrogen‐bond donor ability, and nucleophilicity. The material that contains iodine and is protonated by an inorganic acid shows an excellent catalytic activity for CO <sub>2</sub> conversion into cyclic carbonates with good recyclability. Reaction parameters for the cycloaddition of CO <sub>2</sub> with propylene oxide to propylene carbonate were optimized. The one‐component material is an efficient heterogeneous catalyst for CO <sub>2</sub> cycloaddition reactions and is a greener alternative to conventional supported transition‐metal catalysts. Its catalytic features were also compared to those of the unsupported free ionic compound and other supported catalysts reported previously. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 支持的两性离子纳米粒子的使用是新公司发展的有趣和重要策略 <sub> 2 </ sub> 转化催化剂具有增强的活性和选择性。通过使用FTIR光谱，固态NMR光谱，X射线光电子能谱，XRD，TEM和热重分析，制备桥接介孔杂交二氧化硅材料的几种二十羟基咪唑 - 尿素衍生物框架。新的im-si-x-？材料具有高表面积，氢键供体能和亲核性。含有碘的材料并由无机酸质子化显示出具有优异的CO的催化活性 <sub> 2 </ sub> 转化为具有良好可回收性的循环碳酸盐。 CO的环形加成的反应参数 <sub> 2 </ sub> 优化环氧丙基丙烷丙烯。单组分材料是有效的有效的异质催化剂 <sub> 2 </ sub> 环加成反应，是传统支持的过渡金属催化剂的更绿色替代品。其催化特征也与未浮相的游离离子化合物和先前报道的其它负载型催化剂相比。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16041/'>《ChemCatChem》</a> <b style="margin: 0 2px;">|</b><span>2018年第8期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=cycloaddition&option=203" rel="nofollow">cycloaddition;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=heterogeneous catalysis&option=203" rel="nofollow">heterogeneous catalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogen bonds&option=203" rel="nofollow">hydrogen bonds;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoparticles&option=203" rel="nofollow">nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=zwitterions&option=203" rel="nofollow">zwitterions;</a> </p> <div class="translation"> 机译：环加成;异质催化;氢键;纳米颗粒;两包; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022059382.html">Zwitterionic Imidazole‐Urea Derivative Framework Bridged Mesoporous Hybrid Silica: A Highly Efficient Heterogeneous Nanocatalyst for Carbon Dioxide Conversion</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> </a> <a href="/journal-foreign-16041/" target="_blank" rel="nofollow" class="tuijian_authcolor">ChemCatChem .</a> <span>2018</span><span>,第8期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：两性离子咪唑 - 尿素衍生物框架桥接介孔杂交二氧化硅：用于二氧化碳转化的高效非均相纳米催化剂</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704021713764.html">Isocyanurate-based periodic mesoporous organosilica (PMO-ICS): a highly efficient and recoverable nanocatalyst for the one-pot synthesis of substituted imidazoles and benzimidazoles</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dekamin Mohammad G.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dekamin Mohammad G.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Arefi Elham&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Arefi Elham,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yaghoubi Amene&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yaghoubi Amene </a> <a href="/journal-foreign-27299/" target="_blank" rel="nofollow" class="tuijian_authcolor">RSC Advances .</a> <span>2016</span><span>,第90期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：基于异氰脲酸酯的周期性介孔有机溶胶（PMO-IC）：一种高效且可回收的纳米催化剂，用于单粒子合成取代的咪唑和苯并咪唑</span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_detail_thesis/0204121346093.html">Isocyanurate-based periodic mesoporous organosilica (PMO-ICS): a highly efficient and recoverable nanocatalyst for the one-pot synthesis of substituted imidazoles and benzimidazoles</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mohammad G. 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Qi Sun</a> <span> . 2018</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061202356661.html">一种胺基功能化介孔二氧化硅微球负载型非均相催化剂及制备方法与应用</a> <b>[P]</b> . <span> 中国专利： CN104741140B </span> <span> . 2017.03.01</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120107221047.html">一种胺基功能化介孔二氧化硅微球负载型非均相催化剂及制备方法与应用</a> <b>[P]</b> . <span> 中国专利： CN104741140A </span> <span> . 2015-07-01</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130400632042.html">Method for preparation of mesoporous silica form from power plant fly ash and carbon dioxide sorbents or rare earth metals ion collector based on mesoporous silica form prepared by the method</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR102096364B1 </span> <span> . 2020-04-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：由发电厂的粉煤灰和二氧化碳吸附剂或稀土金属离子收集器制备介孔二氧化硅的方法，所述方法基于该方法制备的介孔二氧化硅 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130400775560.html">Method for preparation of mesoporous silica form from power plant fly ash and carbon dioxide sorbents or rare earth metals ion collector based on mesoporous silica form prepared by the method</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR20200016527A </span> <span> . 2020-02-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：由发电厂的粉煤灰和二氧化碳吸附剂或稀土金属离子收集器制备介孔二氧化硅的方法，所述方法基于该方法制备的介孔二氧化硅 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130422091933.html">METHOD FOR PREPARATION OF ZEOLITE 13X AND MESOPOROUS SILICA DERIVED FROM POWER PLANT BOTTOM ASH, AND CARBON DIOXIDE SORBENTS BASED ON ZEOLITE 13X AND MESOPOROUS SILICA PREPARED BY THE METHOD</a> <b>[P]</b> . <span> 外国专利： <!-- 韩国专利： --> KR20120007882A </span> <span> . 2012-01-25</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：一种由电厂底部灰分衍生的沸石13x和中孔二氧化硅的制备方法，以及基于该方法制备的基于沸石13x和中孔二氧化硅的二氧化碳吸附剂 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022059382','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div 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