Photocatalytic Hydrogen Production: A Rift into the Future Energy Supply

摘要

Abstract > Photocatalytic hydrogen (H <sub>2</sub> ) production is a process that converts solar energy into chemical energy by means of a suitable photocatalyst. After the huge amount of systems that have been tested in the last forty years, the advent of nanotechnology and a careful design at molecular level, allow to obtain attractive activity, even using pure visible light. At the same time we are approaching reasonable photocatalyst stability in laboratory test, and the attention is paid to identify cost‐effective photocatalysts that might find real applications. This Review provides a broad overview of the elementary steps of the heterogeneous photocatalytic H <sub>2</sub> production, including an outline of the physico‐chemical reactions occurring on semiconductors and cocatalysts. The use of different renewable oxygenates as sustainable sacrificial agent for the H <sub>2</sub> production is outlined, in view of a transition from fossil fuels to pure water splitting. Finally, the recent advances in the development of photocatalyst are discussed focusing on the current progress in organic and hybrid organic/inorganic photocatalysts. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 光催化氢气（H. <sub> 2 </ sub> ）生产是通过合适的光催化剂将太阳能转化为化学能的过程。在过去的四十年中已经测试过大量的系统之后，纳米技术的出现和分子水平的仔细设计，甚至可以获得有吸引力的活动，甚至使用纯可见光。与此同时，我们在实验室测试中接近合理的光催化稳定性，并且需要注意的是识别可能找到真实应用的经济高效的光催化剂。本综述提供了异质光催化H的基本步骤的广泛概述 <sub> 2 </ sub> 生产，包括在半导体和助催化剂上发生的物理化学反应的概要。使用不同的可再生含氧化合物作为H的可持续牺牲剂 <sub> 2 </ sub> 考虑到从化石燃料到纯净的水分裂的过渡，生产了生产。最后，讨论了光催化剂的开发的最近进步，重点是有机和杂交有机/无机光催化剂的目前进展。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16041/'>《ChemCatChem 》</a> <b style="margin: 0 2px;">|</b><span>2017年第9期</span><b style="margin: 0 2px;">|</b> <span>共22页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogen&option=203" rel="nofollow">hydrogen;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photocatalysis&option=203" rel="nofollow">photocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photoreforming&option=203" rel="nofollow">photoreforming;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=renewable energy&option=203" rel="nofollow">renewable energy;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=water splitting&option=203" rel="nofollow">water splitting;</a> </p> <div class="translation"> 机译：氢气;光催化;光致态;可再生能量;水分裂; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022059202.html">Photocatalytic Hydrogen Production: A Rift into the Future Energy Supply</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> </a> <a href="/journal-foreign-16041/" target="_blank" rel="nofollow" class="tuijian_authcolor">ChemCatChem .</a> <span>2017</span> <span>,第9期</span> </span> </div> <p class="zwjiyix 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carbon fiber with a safety valve for use in grafting instantaneous circuit on new electric vehicles in double energy to supply fast grandi numbers daily car, in order to provide broad autonomy to obtain the complete autonomy of supply with spare cylinders.with a network of service stations with high thermal insulation flame-retardant simplified and noise, without need of public land for parking.for the production and storage in the small space of large amounts of electrolyte hydrogen produced with renewable energy.for their use in the automotive and the rehabilitation of the environment through the use of electrolytic water in place of oil. they form a comprehensive integrated system of electric mobilitydual energy range extender to hydrogen.</a> <b>[P]</b> . <span> 外国专利：  ITUA20161289A1 </span> <span> . 2017-08-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：带有安全阀的移动式碳纤维可互换钢瓶，用于双能量接枝到新的电动汽车的瞬时电路上，为日用车提供快速重数供应，以提供广泛的自治权，从而获得备用钢瓶的完全供应权。加油站网络，具有极高的隔热性，阻燃性和简化性，无需公共土地停放。用于在小空间中生产和储存大量可再生能源产生的电解质氢，用于汽车和通过使用电解水代替油来恢复环境。它们形成了电动势的综合集成系统-将能量扩展为氢。 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130443684770.html">Photocatalytic element for decomposing hydrogen-containing compounds, especially for supplying hydrogen to fuel cells, comprises a thin photocatalytic layer on a support with an open pore structure</a> <b>[P]</b> . <span> 外国专利：  DE10210465A1 </span> <span> . 2003-10-09</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于分解含氢化合物，特别是用于向燃料电池供应氢的光催化元件，包括在具有开放孔结构的载体上的薄光催化层 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130500811506.html">CATALYST FOR THE PHOTOCATALYTIC PRODUCTION OF HYDROGEN, A METHOD FOR ITS PREPARATION AND A METHOD FOR THE PHOTOCATALYTIC PRODUCTION OF HYDROGEN</a> <b>[P]</b> . <span> 外国专利：  RU2757277C1 </span> <span> . 2021-10-12</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：氢催化剂的催化剂，其制备方法及其制备方法及其光催化生产氢气 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704022059202','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img 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