Decline in Antarctic Ozone Depletion and Lower Stratospheric Chlorine Determined From Aura Microwave Limb Sounder Observations

Strahan Susan E.; Douglass Anne R.

摘要

Abstract > Attribution of Antarctic ozone recovery to the Montreal protocol requires evidence that (1) Antarctic chlorine levels are declining and (2) there is a reduction in ozone depletion in response to a chlorine decline. We use Aura Microwave Limb Sounder measurements of O <sub>3</sub> , HCl, and N <sub>2</sub> O to demonstrate that inorganic chlorine (Cl <sub>y</sub> ) from 2013 to 2016 was 223?±?93?parts per trillion lower in the Antarctic lower stratosphere than from 2004 to 2007 and that column ozone depletion declined in response. The mean Cl <sub>y</sub> decline rate, ~0.8%/yr, agrees with the expected rate based on chlorofluorocarbon lifetimes. N <sub>2</sub> O measurements are crucial for identifying changes in stratospheric Cl <sub>y</sub> loading independent of dynamical variability. From 2005 to 2016, the ozone depletion and Cl <sub>y</sub> time series show matching periods of decline, stability, and increase. The observed sensitivity of O <sub>3</sub> depletion to changing Cl <sub>y</sub> agrees with the sensitivity simulated by the Global Modeling Initiative chemistry transport model integrated with Modern Era Retrospective Analysis for Research and Applications 2 meteorology. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>摘要</ title> >南极臭氧恢复到蒙特利尔方案需要证据表明（1）南极氯水平衰退和（2）臭氧耗竭减少，响应氯衰退。我们使用O <sub> 3 </ sub>，HCl和N <sub> 2 </ sub> O的Aura微波肢体测量仪测量，以证明2013年的无机氯（CL <sub> Y </ sub>） 2016年是223？±93？南极较低平流层每万亿的零件比2004年至2007年较低，漏斗耗竭率下降。平均cl <sub> y </ sub>下降率，〜0.8％/ yr，同意基于氯氟烃寿命的预期速率。 n <sub> 2 </ sub> o测量对于识别与动力学变异性无关的平流层CL <sub> y </ sub>负载的变化至关重要。从2005年到2016年，臭氧耗尽和CL <Sub> Y </ Sub>时间序列显示匹配期的下降，稳定性和增加。观察到的O <sub> 3 </ sub>耗尽到改变CL <sub> y </ sub>的敏感性，同意全球建模倡议化学传输模型模拟的灵敏度与现代时代回顾性分析进行研究和应用2气象学。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-23539/'>《Geophysical Research Letters》</a> <b style="margin: 0 2px;">|</b><span>2018年第1期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Strahan Susan E.&option=202" target="_blank" rel="nofollow">Strahan Susan E.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Douglass Anne R.&option=202" target="_blank" rel="nofollow">Douglass Anne R.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Universities Space Research AssociationColumbia MD USA;</p> <p>Atmospheric Chemistry and Dynamics LaboratoryNASA Goddard Space Flight CenterGreenbelt MD USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Antarctic ozone&option=203" rel="nofollow">Antarctic ozone;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ozone recovery&option=203" rel="nofollow">ozone recovery;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ozone depletion&option=203" rel="nofollow">ozone depletion;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ozone depleting substances&option=203" rel="nofollow">ozone depleting substances;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=inorganic chlorine&option=203" rel="nofollow">inorganic chlorine;</a> </p> <div class="translation"> 机译：南极臭氧;臭氧恢复;臭氧消耗;臭氧耗尽物质;无机氯; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704019850924.html">Decline in Antarctic Ozone Depletion and Lower Stratospheric Chlorine Determined From Aura Microwave Limb Sounder Observations</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Strahan Susan E.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Strahan Susan E.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Douglass Anne R.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Douglass Anne R. </a> <a href="/journal-foreign-23539/" target="_blank" rel="nofollow" class="tuijian_authcolor">Geophysical Research Letters .</a> <span>2018</span><span>,第1期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：南极臭氧耗竭和低于光环微波肢体探测器观测测定的南极臭氧耗竭和较低的划分氯</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_detail_thesis/0204114967799.html">A Match-based approach to the estimation of polar stratospheric ozone loss using Aura Microwave Limb Sounder observations</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Livesey N. 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