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Nonequilibrium Dynamics in Amorphous Si_3b_3n_7

机译:非晶Si_3b_3n_7中的非平衡动力学

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摘要

We present extensive numerical investigations of the structural relaxation dynamics of a realistic model of the amorphous high-temperature ceramic alpha-Si_3b_3n_7,probing the mean-square displacement of the atoms,the bond survival probability,the average energy,the specific heat,and the two-point energy average.Combining the information from these different sources,we identify a transition temperature T_c approx= 2000 K below which the system is no longer ergodic and physical quantities observed over a time t_(obs)show a systematic parametric dependence on the waiting time t_w,or age,elapsed after the quench.The aging dynamics "stiffens" as the system becomes older,which is similar to the behavior of highly idealized models such as Ising spin glasses and Lennard-Jones glasses.
机译:我们对非晶态高温陶瓷alpha-Si_3b_3n_7的逼真的模型的结构弛豫动力学进行了广泛的数值研究,探索了原子的均方位移,键的存活率,平均能量,比热和两点平均能量。结合来自这些不同来源的信息,我们确定过渡温度T_c大约= 2000 K,低于该温度时系统不再是遍历遍历,并且在时间t_(obs)上观察到的物理量显示出对参数的系统性参数依赖性。淬火后经过的等待时间t_w或年龄。随着系统的变老,老化动力学会“变硬”,这与高度理想化的模型(例如Ising旋转眼镜和Lennard-Jones眼镜)的行为类似。

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