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首页> 外文期刊>The Journal of Chemical Physics >Electromagnetic fluctuation-induced interactions in randomly charged slabs
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Electromagnetic fluctuation-induced interactions in randomly charged slabs

机译:电磁感应在随机带电平板中的相互作用

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摘要

Randomly charged net-neutral dielectric slabs are shown to interact across a featureless dielectric continuum with long-range electrostatic forces that scale with the statistical variance of their quenched random charge distribution and inversely with the distance between their bounding surfaces. By accounting for the whole spectrum of electromagnetic field fluctuations, we show that this long-range disorder-generated interaction extends well into the retarded regime where higher order (non-zero) Matsubara frequencies contribute significantly. This occurs even for highly clean samples with only a trace amount of charge disorder and shows that disorder effects can be important down to the nanoscale. As a result, the previously predicted non-monotonic behavior for the total force between dissimilar slabs as a function of their separation distance is substantially modified by higher order contributions, and in almost all cases of interest, we find that the equilibrium inter-surface separation is shifted to substantially larger values compared to predictions based solely on the zero-frequency component. This suggests that the ensuing non-monotonic interaction is more easily amenable to experimental detection. The presence of charge disorder in the intervening dielectric medium between the two slabs is shown to lead to an additional force that can be repulsive or attractive depending on the system parameters and can, for instance, wash out the non-monotonic behavior of the total force when the intervening slab contains a sufficiently large amount of disorder charges.
机译:随机带电的中性电介质平板显示为在无特征的电介质连续体上相互作用,并具有远距离静电力,该静电力随其淬灭的随机电荷分布的统计方差以及与其边界表面之间的距离成反比而缩放。通过考虑电磁场波动的整个频谱,我们表明,这种由远程无序产生的相互作用很好地扩展到了延迟状态,在延迟状态中,高阶(非零)松原频率显着起作用。即使对于只有极少量电荷无序的高度清洁的样品,也会发生这种情况,这表明低至纳米级的无序效应可能很重要。结果,先前预测的不同板之间总力作为其分离距离的函数的非单调行为被较高阶的贡献大大地改变,并且在几乎所有感兴趣的情况下,我们发现平衡的表面间分离与仅基于零频率分量的预测相比,α偏移到实质上更大的值。这表明随后发生的非单调相互作用更易于进行实验检测。结果表明,在两个平板之间的介电介质中存在电荷无序会导致产生附加力,该附加力根据系统参数可能是排斥的或有吸引力的,并且例如可以冲刷总力的非单调行为。当中间板包含足够数量的无序电荷时。

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