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Unidirectional hopping transport of interacting particles on a finite chain

机译:有限链上相互作用粒子的单向跳跃传输

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摘要

Particle transport through an open, discrete one-dimensional channel against a mechanical or chemical bias is analyzed within a master equation approach. The channel, externally driven by time-dependent site energies, allows multiple occupation due to the coupling to reservoirs. Performance criteria and optimization of active transport in a two-site channel are discussed as a function of reservoir chemical potentials, the load potential, interparticle interaction strength, driving mode, and driving period. Our results, derived from exact rate equations, are used in addition to test a previously developed time-dependent density functional theory, suggesting a wider applicability of that method in investigations of many particle systems far from equilibrium.
机译:在主方程方法中分析了通过机械离散或化学偏置通过开放的离散一维通道进行的粒子传输。该通道由与时间有关的位置能量从外部驱动,由于与储层耦合,因此可以进行多次占领。根据储层化学势,负荷势,颗粒间相互作用强度,驱动方式和驱动周期,讨论了在两个站点通道中的性能标准和主动输运的优化。我们的结果源自精确的速率方程,此外还用于测试先前开发的随时间变化的密度泛函理论,表明该方法在研究许多远离平衡的粒子系统时具有更广泛的适用性。

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